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  Self-healing response in supramolecular polymers based on reversible zinc–histidine interactions

Enke, M., Bode, S., Vitz, J., Schacher, F. H., Harrington, M. J., Hager, M. D., et al. (2015). Self-healing response in supramolecular polymers based on reversible zinc–histidine interactions. Polymer, 69, 274-282. doi:10.1016/j.polymer.2015.03.068.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0028-285A-8 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0028-285C-4
Genre: Journal Article

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 Creators:
Enke, Marcel, Author
Bode, Stefan, Author
Vitz, Jürgen, Author
Schacher, Felix H., Author
Harrington, Matthew J.1, Author              
Hager, Martin D., Author
Schubert, Ulrich S., Author
Affiliations:
1Matthew Harrington, Biomaterialien, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863292              

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Free keywords: Self-healing polymers
 Abstract: Abstract Histidine-metal interactions are utilized in many biological materials as reinforcing crosslinks, and in particular, are believed to contribute as reversible crosslinks to the intrinsic self-recovery behavior of mussel byssal threads. In this contribution, two new histidine-based monomers were synthesized and further copolymerized with butyl methacrylate (BMA) and lauryl methacrylate (LMA) applying the reversible addition–fragmentation chain transfer (RAFT) polymerization technique. Crosslinking with zinc ions resulted in supramolecular metallopolymer networks exhibiting a self-healing behavior that was tunable depending on the specific zinc salt used. The presented results provide a class of new polymeric species with different self-healing capacities.

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 Dates: 2015-04-012015-07-09
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.1016/j.polymer.2015.03.068
BibTex Citekey: Enke2015274
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Title: Polymer
  Other : Polymer
Source Genre: Journal
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Publ. Info: Guildford, England : Elsevier
Pages: - Volume / Issue: 69 Sequence Number: - Start / End Page: 274 - 282 Identifier: ISSN: 0032-3861
CoNE: https://pure.mpg.de/cone/journals/resource/954925434439