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  Multiple-quantum excitation probabilities of Einstein-like modes of surface adsorbates induced by He-atom scattering

Manson, J. R., Graham, A. P., & Li, M. B. (2002). Multiple-quantum excitation probabilities of Einstein-like modes of surface adsorbates induced by He-atom scattering. Journal of Physics-Condensed Matter, 14(24), 6233-6261.

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Datensatz-Permalink: https://hdl.handle.net/11858/00-001M-0000-0029-1773-6 Versions-Permalink: https://hdl.handle.net/11858/00-001M-0000-0029-1774-4
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 Urheber:
Manson, J. R., Autor
Graham, A. P.1, Autor           
Li, M. B., Autor
Affiliations:
1Emeritus Group Molecular Interactions, Max Planck Institute for Dynamics and Self-Organization, Max Planck Society, ou_2063297              

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 Zusammenfassung: Experimental data exhibiting multiple-quantum excitation of the vibrational modes of decoupled, oscillating adsorbates on a surface via impact by a He atom are reviewed for the cases of carbon monoxide and heavy rare gases adsorbed on metal substrates. The experimental scattering spectra are analysed using a dynamical scattering model that predicts correctly the angular dependences of the distributions of multiphonon excitations and the variation with incident energy and adsorbate frequency. The agreement between experiment and theory indicates that the details of the He-surface interaction potential are relatively unimportant for incident energies much higher than the vibrational energy. The model is used to predict the excitation probabilities of other possible vibrational modes which have not yet been observed using helium-atom scattering.

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Sprache(n): eng - English
 Datum: 2002-06-24
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: eDoc: 13445
ISI: 000176726100019
 Art des Abschluß: -

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Titel: Journal of Physics-Condensed Matter
  Alternativer Titel : J. Phys.-Condes. Matter
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: -
Seiten: - Band / Heft: 14 (24) Artikelnummer: - Start- / Endseite: 6233 - 6261 Identifikator: ISSN: 0953-8984