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  Isomerization and melting-like transition of size-selected water nonamers

Brudermann, J., Buck, U., & Buch, V. (2002). Isomerization and melting-like transition of size-selected water nonamers. Journal of Physical Chemistry A, 106(3), 453-457.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0029-17A5-3 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0029-17A6-1
Genre: Journal Article

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 Creators:
Brudermann, J.1, Author              
Buck, U.1, Author              
Buch, V., Author
Affiliations:
1Research Group Clusterdynamik, Max Planck Institute for Dynamics and Self-Organization, Max Planck Society, ou_2063296              

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 Abstract: The vibrational OH-stretch spectra of size-selected pure water (H2O)9 clusters, measured at two different temperatures, have been used to identify isomeric transitions. The broad, featureless high-temperature, liquid-like spectrum resembles that of water, while the structured low- temperature, solid- like spectrum differs appreciably from that of ice. Accompanying calculations suggest that the low-temperature spectra originate from two cube-like structures. The high temperature spectra appear to be above an isomeric transition to more open amorphous arrangements of fused three- to five- membered rings.

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Language(s): eng - English
 Dates: 2002-01-24
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Method: -
 Identifiers: eDoc: 13461
ISI: 000173356100001
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Title: Journal of Physical Chemistry A
  Alternative Title : J. Phys. Chem. A
Source Genre: Journal
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Pages: - Volume / Issue: 106 (3) Sequence Number: - Start / End Page: 453 - 457 Identifier: ISSN: 1089-5639