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  The nonlinear response of stratospheric ozone to NOx and ClOx perturbations

Yang, P., & Brasseur, G. P. (2001). The nonlinear response of stratospheric ozone to NOx and ClOx perturbations. Gophysical Research Letters, 28, 717-720. doi:10.1029/2000GL011428.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0029-0221-1 Version Permalink: http://hdl.handle.net/21.11116/0000-0003-006F-1
Genre: Journal Article

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Yang_et_al-2001-Geophysical_Research_Letters.pdf (Publisher version), 509KB
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 Creators:
Yang, P.C.1, Author
Brasseur, Guy P.2, Author              
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1external, ou_persistent22              
2The Atmosphere in the Earth System, MPI for Meteorology, Max Planck Society, ou_913550              

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 Abstract: A mathematical analysis of the stratospheric photochemical system (gas phase reactions only) shows the existence of potential catastrophe mechanisms which could produce a dramatic reduction in the ozone concentration near 25 km altitude. The conditions leading to such catastrophe correspond to a relatively modest (i.e., factor 2-2.5) increase in the stratospheric source of reactive nitrogen (NOx). For a tenfold increase in the source of reactive chlorine (ClOx), the ozone system exhibits a large amplitude oscillatory behavior with a period of several tens of years. Transport processes could, however, damp these dramatic changes resulting from the nonlinear nature of the stratospheric chemical system.

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Language(s): eng - English
 Dates: 2001-02-15
 Publication Status: Published in print
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 Rev. Type: Peer
 Identifiers: ISI: 000166916500041
DOI: 10.1029/2000GL011428
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Title: Gophysical Research Letters
Source Genre: Journal
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Pages: - Volume / Issue: 28 Sequence Number: - Start / End Page: 717 - 720 Identifier: ISSN: 0094-8276