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  On the relation between population kinetics and state-to-state rate coefficients for vibrational energy transfer.

Dashevskaya, E., Litvin, I., & Nikitin, E. E. (2015). On the relation between population kinetics and state-to-state rate coefficients for vibrational energy transfer. Zeitschrift für Physikalische Chemie, 229(10-12), 1561-1574. doi:10.1515/zpch-2015-0597.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0029-1D28-9 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-7475-0
Genre: Journal Article

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 Creators:
Dashevskaya, E.I.1, Author              
Litvin, I.1, Author              
Nikitin, E. E.1, Author              
Affiliations:
1Emeritus Group of Spectroscopy and Photochemical Kinetics, MPI for Biophysical Chemistry, Max Planck Society, ou_578625              

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Free keywords: Reaction kinetics
 Abstract: The relation between time-dependent population of vibrational state and collision-induced state-to-state rate coefficients is discussed within the Landau–Teller kinetic equations for the relaxation of harmonic oscillators in a heat bath. In particular, the increase of the populations in the first and the second vibrational state of an initially cold oscillator shows a considerable variety of its relation to a single Landau–Teller state-to-state rate coefficient. It is suggested that this variety should be kept in mind when experimental studies of the relaxation of specific level are analyzed.

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Language(s): eng - English
 Dates: 2015-09-282015-10
 Publication Status: Published in print
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 Rev. Method: Peer
 Identifiers: DOI: 10.1515/zpch-2015-0597
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Title: Zeitschrift für Physikalische Chemie
Source Genre: Journal
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Pages: - Volume / Issue: 229 (10-12) Sequence Number: - Start / End Page: 1561 - 1574 Identifier: -