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Zusammenfassung:
The seasonal variability of black carbon (BC) aerosols in India is studied using high resolution (10 km) BC simulations conducted using the Weather Research and Forecasting Model coupled with Chemistry. The model reproduces the observed seasonality of surface BC fairly well over most parts of India but fails to capture the seasonality in the Himalayas and deviates from the observed BC magnitude at several sites. The errors in modeled BC are attributed to uncertainties in BC emissions and their diurnal cycle, planetary boundary layer height underestimation, and aerosol processes. Model results show distinct but opposite seasonality of BC in the lower (LT) and free troposphere (FT) with BC showing winter maximum and summer minimum in the LT and vice versa in the FT. Our analysis shows that BC seasonality is not driven by seasonality of the anthropogenic emissions but by changes in the regional meteorology through weakening of the horizontal transport and strengthening of the vertical transport of BC during summertime compared to winter. BC in both the LT and FT comes mostly from anthropogenic emissions followed by biomass burning emissions except during winter when long-distant sources become more important in the FT. BC in the FT is significantly affected by anthropogenic emissions from all parts of India. The source-receptor relationship changes seasonally, but the regional transport remains a significant contributor to BC loadings in the LT of India, highlighting the necessity of considering nonlocal sources along with local emissions when designing strategies for mitigating BC impacts on air quality.
