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  Comprehensive mapping and characteristic regimes of aerosol effects on the formation and evolution of pyro-convective clouds

Chang, D., Cheng, Y., Reutter, P., Trentmann, J., Burrows, S. M., Spichtinger, P., Nordmann, S., Andreae, M. O., Pöschl, U., & Su, H. (2015). Comprehensive mapping and characteristic regimes of aerosol effects on the formation and evolution of pyro-convective clouds. Atmospheric Chemistry and Physics, 15(18), 10325-10348. doi:10.5194/acp-15-10325-2015.

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資料種別: 学術論文

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 作成者:
Chang, D.1, 著者           
Cheng, Y.1, 著者           
Reutter, P.2, 著者
Trentmann, J.2, 著者
Burrows, S. M.2, 著者
Spichtinger, P.2, 著者
Nordmann, S.1, 著者           
Andreae, M. O.3, 著者           
Pöschl, U.1, 著者           
Su, H.1, 著者           
所属:
1Multiphase Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826290              
2external, ou_persistent22              
3Biogeochemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826286              

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 要旨: A recent parcel model study (Reutter et al., 2009) showed three deterministic regimes of initial cloud droplet formation, characterized by different ratios of aerosol concentrations (N-CN) to updraft velocities. This analysis, however, did not reveal how these regimes evolve during the subsequent cloud development. To address this issue, we employed the Active Tracer High Resolution Atmospheric Model (ATHAM) with full microphysics and extended the model simulation from the cloud base to the entire column of a single pyro-convective mixed-phase cloud. A series of 2-D simulations (over 1000) were performed over a wide range of N-CN and dynamic conditions. The integrated concentration of hydrometeors over the full spatial and temporal scales was used to evaluate the aerosol and dynamic effects. The results show the following. (1) The three regimes for cloud condensation nuclei (CCN) activation in the parcel model (namely aerosol-limited, updraft-limited, and transitional regimes) still exist within our simulations, but net production of raindrops and frozen particles occurs mostly within the updraft-limited regime. (2) Generally, elevated aerosols enhance the formation of cloud droplets and frozen particles. The response of raindrops and precipitation to aerosols is more complex and can be either positive or negative as a function of aerosol concentrations. The most negative effect was found for values of N-CN of similar to 1000 to 3000 cm(-3). (3) The nonlinear properties of aerosol-cloud interactions challenge the conclusions drawn from limited case studies in terms of their representativeness, and ensemble studies over a wide range of aerosol concentrations and other influencing factors are strongly recommended for a more robust assessment of the aerosol effects.

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 日付: 2015
 出版の状態: 出版
 ページ: -
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 識別子(DOI, ISBNなど): ISI: 000362457400007
DOI: 10.5194/acp-15-10325-2015
 学位: -

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出版物 1

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出版物名: Atmospheric Chemistry and Physics
種別: 学術雑誌
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出版社, 出版地: Katlenburg-Lindau, Germany : European Geosciences Union
ページ: - 巻号: 15 (18) 通巻号: - 開始・終了ページ: 10325 - 10348 識別子(ISBN, ISSN, DOIなど): ISSN: 1680-7316
CoNE: https://pure.mpg.de/cone/journals/resource/111030403014016