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  Early stages of glacial clustering in supercooled triphenyl phosphite

Schwickert, B. E., Kline, S. R., Zimmermann, H., Lantzky, K. M., & Yarger, J. L. (2001). Early stages of glacial clustering in supercooled triphenyl phosphite. Physical Review B, 64, 405-410. doi:10.1103/PhysRevB.64.045410.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0029-222B-F Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0029-222C-D
Genre: Journal Article
Alternative Title : Early stages of glacial clustering in supercooled triphenyl phosphite

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PhysRevB_64_2001_045410e.pdf (Any fulltext), 161KB
 
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http://journals.aps.org/prb/pdf/10.1103/PhysRevB.64.045410 (Any fulltext)
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http://dx.doi.org/10.1103/PhysRevB.64.045410 (Any fulltext)
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 Creators:
Schwickert, Birgit Effey, Author
Kline, Steven R., Author
Zimmermann, Herbert1, 2, Author           
Lantzky, K. M., Author
Yarger, Jeffery L., Author
Affiliations:
1Department of Molecular Physics, Max Planck Institute for Medical Research, Max Planck Society, ou_1497705              
2Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              

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 Abstract: Glacial phase clustering and growth in triphenyl phosphite is observed in the temperature interval of 210 K to 214 K by small angle neutron scattering performed at the NIST Center for Neutron Research. Presented are the radius, volume fraction, and polydispersity of clusters of glacial phase surrounded by a supercooled liquid. The data can be interpreted in a four-step model of (I) cluster formation, (II) rapid nucleation, (III) agglomeration, and finally (IV) saturation. Two schemes of cluster growth can be identified. The first one is a region of radius stagnation (II), which is followed by a region of volume stagnation (III). Competition between the increase in cluster size and the increase in the number of clusters is deduced from this behavior.

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Language(s): eng - English
 Dates: 2001-01-212000-10-252001-01-242001-07-02
 Publication Status: Issued
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: eDoc: 666205
DOI: 10.1103/PhysRevB.64.045410
Other: 5012
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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: - Volume / Issue: 64 Sequence Number: - Start / End Page: 405 - 410 Identifier: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008