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  Using ion imaging to measure velocity distributions in surface scattering experiments.

Harding, D. J., Neugebohren, J., Auerbach, D. J., Kitsopoulos, T. N., & Wodtke, A. M. (2015). Using ion imaging to measure velocity distributions in surface scattering experiments. Journal of Physical Chemistry A, 119(50), 12255-12262. doi:10.1021/acs.jpca.5b06272.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0029-48F0-E Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002A-1106-A
Genre: Journal Article

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Harding, D. J.1, Author              
Neugebohren, J.1, Author              
Auerbach, D. J.1, Author              
Kitsopoulos, T. N.1, Author              
Wodtke, A. M.1, Author              
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1Department of Dynamics at Surfaces, MPI for Biophysical Chemistry, Max Planck Society, ou_578600              

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 Abstract: We present a new implementation of ion imaging for the study of surface scattering processes. The technique uses a combination of spatial ion imaging with laser slicing and delayed pulsed extraction. The scattering velocities of interest are parallel to the imaging plane, allowing speed and angular distributions to be extracted from a single image. The first results of direct scattering of N-2 from a clean, single-crystal Au(111) surface are reported, and the speed resolution is shown to be competitive with current state-of-the-art time-of-flight methods for velocity measurements while providing simultaneous measurements of in-plane angular distributions.

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Language(s): eng - English
 Dates: 2015-09-292015-12-17
 Publication Status: Published in print
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 Rev. Method: Peer
 Identifiers: DOI: 10.1021/acs.jpca.5b06272
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Title: Journal of Physical Chemistry A
Source Genre: Journal
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Pages: - Volume / Issue: 119 (50) Sequence Number: - Start / End Page: 12255 - 12262 Identifier: -