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  Mild Continuous Hydrogenolysis of Kraft Lignin over Titanium Nitride-Nickel Catalyst

Molinari, V., Clavel, G., Graglia, M., Antonietti, M., & Esposito, D. (2016). Mild Continuous Hydrogenolysis of Kraft Lignin over Titanium Nitride-Nickel Catalyst. ACS Catalysis, 6(3), 1663-1670. doi:10.1021/acscatal.5b01926.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0029-7D29-5 Version Permalink: http://hdl.handle.net/21.11116/0000-0005-DD1F-1
Genre: Journal Article
Alternative Title : ACS Catalysis

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 Creators:
Molinari, Valerio1, Author              
Clavel, Guylhaine2, Author              
Graglia, Micaela1, Author              
Antonietti, Markus3, Author              
Esposito, Davide1, Author              
Affiliations:
1Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863315              
2Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              
3Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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 Abstract: Lignin is one of the most important candidates for the procurement of renewable aromatics. The development of successful strategies for the production of building blocks from lignin implies the design of effective depolymerisation protocols. Here we propose a continuous flow approach for the hydrogenolysis of kraft lignin utilizing a TiN-Ni heterogeneous catalyst. The refining of commercial kraft lignin was evaluated, showing that the catalyst can facilitate the partial depolymerisation of this sulfur containing material under very mild conditions and short residence times. The process restitutes lignin in the form of oligomers in combination with an array of valuable single-ring aromatic compounds.

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 Dates: 2016-01-262016
 Publication Status: Published in print
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 Identifiers: DOI: 10.1021/acscatal.5b01926
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Title: ACS Catalysis
  Abbreviation : ACS Catal.
Source Genre: Journal
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Publ. Info: Washington, DC : ACS
Pages: - Volume / Issue: 6 (3) Sequence Number: - Start / End Page: 1663 - 1670 Identifier: ISSN: 2155-5435