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  A broad supersaturation scanning (BS2) approach for rapid measurement of aerosol particle hygroscopicity and cloud condensation nuclei activity

Su, H., Cheng, Y., Wang, Z., Pöhlker, C., Nillius, B., Wiedensohler, A., & Pöschl, U. (2015). A broad supersaturation scanning (BS2) approach for rapid measurement of aerosol particle hygroscopicity and cloud condensation nuclei activity. Atmospheric Measurement Techniques Discussions, 8, 9713-9730. doi:10.5194/amtd-8-9713-2015.

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資料種別: 成果報告書

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 作成者:
Su, H.1, 著者           
Cheng, Y.1, 著者           
Wang, Z.1, 著者           
Pöhlker, C.2, 著者           
Nillius, Björn, 著者
Wiedensohler, A., 著者
Pöschl, U.1, 著者           
所属:
1Multiphase Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826290              
2Biogeochemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826286              

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 要旨: The activation and hygroscopicity of cloud condensation nuclei (CCN) are key to understand aerosol–cloud interactions and their climate impact. It can be measured by scanning the particle size and supersaturation in CCN measurements. The scanning of supersaturation is often time-consuming and limits the temporal resolution and performance of CCN measurements. Here we present a new approach, termed broad supersaturation scanning (BS2) method, in which a range of supersaturation is simultaneously scanned reducing the time interval between different supersaturation scans. The practical applicability of the BS2 approach is demonstrated with nano-CCN measurements of laboratory-generated aerosol particles. Model simulations show that the BS2 approach is also applicable for measuring CCN activation of ambient mixed particles. Due to its fast response and technical simplicity, the BS2 approach may be well suited for long-term measurements. Since hygroscopicity is closely related to the fraction of organics/inorganics in aerosol particles, a BS2-CCN counter can also serve as a complementary sensor for fast detection/estimation of aerosol chemical compositions.

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 日付: 2015-09-17
 出版の状態: オンラインで出版済み
 ページ: 17
 出版情報: -
 目次: -
 査読: -
 識別子(DOI, ISBNなど): DOI: 10.5194/amtd-8-9713-2015
 学位: -

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出版物名: Atmospheric Measurement Techniques Discussions
  その他 : Atmos. Meas. Tech. Discuss.
  省略形 : AMTD
種別: 学術雑誌
 著者・編者:
所属:
出版社, 出版地: Katlenburg-Lindau : Copernicus
ページ: - 巻号: 8 通巻号: - 開始・終了ページ: 9713 - 9730 識別子(ISBN, ISSN, DOIなど): その他: 1867-8610
CoNE: https://pure.mpg.de/cone/journals/resource/1867-8610