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  Vacuum ultraviolet photodissociation of hydrogen bromide.

Su, S., Dorenkamp, Y., Yu, S., Wodtke, A. M., Dai, D., Yuan, K., et al. (2016). Vacuum ultraviolet photodissociation of hydrogen bromide. Physical Chemistry Chemical Physics, 18(22), 15399-15405. doi:10.1039/C6CP01956K.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002A-FFE6-D Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-203D-E
Genre: Journal Article

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Su, S., Author
Dorenkamp, Y.1, Author              
Yu, S., Author
Wodtke, A. M.1, Author              
Dai, D., Author
Yuan, K., Author
Yang, X., Author
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1Department of Dynamics at Surfaces, MPI for Biophysical Chemistry, Max Planck Society, ou_578600              

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 Abstract: Photodissociation dynamics of HBr at a series of photolysis wavelengths in the range of 123.90-125.90 nm and at around 137.0 nm have been studied using the H atom Rydberg "tagging'' time-of-flight technique. The branching fractions between the channels forming ground Br(P-2(3/2)) and spin-orbit excited Br(P-2(1/2)) atoms together with the angular distributions of the products corresponding to these two channels have been measured. The photolysis wavelengths in this work excited the HBr molecule from the ground state X (1)Sigma(+) to various Rydberg states and the V (1)Sigma(+) ion-pair valence state. Predissociation via these states displays rich behavior, indicating the influence of the nature of initially excited states and the coupling to other bound or repulsive states on the predissociation dynamics.

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Language(s): eng - English
 Dates: 2016-05-062016-06-14
 Publication Status: Published in print
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 Rev. Method: Peer
 Identifiers: DOI: 10.1039/C6CP01956K
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Title: Physical Chemistry Chemical Physics
Source Genre: Journal
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Pages: - Volume / Issue: 18 (22) Sequence Number: - Start / End Page: 15399 - 15405 Identifier: -