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  Quantum plasmonics: from jellium models to ab initio calculations

Varas, A., García-González, P., Feist, J., García-Vidal, F. J., & Rubio, A. (2016). Quantum plasmonics: from jellium models to ab initio calculations. Nanophotonics, 5(3), 409-426. doi:10.1515/nanoph-2015-0141.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-1E5F-D Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-A349-A
Genre: Journal Article

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[Nanophotonics] Quantum plasmonics_ from jellium models to ab initio calculations.pdf (Publisher version), 5MB
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[Nanophotonics] Quantum plasmonics_ from jellium models to ab initio calculations.pdf
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2016
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© A. Varas et al.

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http://dx.doi.org/10.1515/nanoph-2015-0141 (Publisher version)
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 Creators:
Varas, Alejandro1, Author
García-González, Pablo2, 3, Author
Feist, Johannes3, Author
García-Vidal, F. J.3, Author
Rubio, Angel1, 4, 5, Author              
Affiliations:
1Nano-Bio Spectroscopy Group and ETSF Scientific Development Centre, Universidad del País Vasco UPV/EHU, CFM CSIC-UPV/EHU, Av. de Tolosa 72, E-20018 Donostia, San Sebastián, Spain, ou_persistent22              
2ETSF Scientific Development Centre, Av. de Tolosa 72, E-20018 Donostia, San Sebastián, Spain, ou_persistent22              
3Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Cantoblanco, Madrid, Spain, ou_persistent22              
4Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
5Center for Free-Electron Laser Science, Luruper Chaussee 149, 22761 Hamburg, Germany, ou_persistent22              

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Free keywords: ab initio methods; plasmonics; nanoparticles; optical absorption; TDDFT
 Abstract: Light-matter interaction in plasmonic nanostructures is often treated within the realm of classical optics. However, recent experimental findings show the need to go beyond the classical models to explain and predict the plasmonic response at the nanoscale. A prototypical system is a nanoparticle dimer, extensively studied using both classical and quantum prescriptions. However, only very recently, fully ab initio time-dependent density functional theory (TDDFT) calculations of the optical response of these dimers have been carried out. Here, we review the recent work on the impact of the atomic structure on the optical properties of such systems. We show that TDDFT can be an invaluable tool to simulate the time evolution of plasmonic modes, providing fundamental understanding into the underlying microscopical mechanisms.

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Language(s): eng - English
 Dates: 2016-01-252015-11-122016-02-292016-09-03
 Publication Status: Published online
 Pages: 18
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1515/nanoph-2015-0141
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Title: Nanophotonics
Source Genre: Journal
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Publ. Info: Berlin, Germany : de Gruyter
Pages: - Volume / Issue: 5 (3) Sequence Number: - Start / End Page: 409 - 426 Identifier: ISSN: 2192-8614
CoNE: https://pure.mpg.de/cone/journals/resource/2192-8614