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  Internal Morphology-Controllable Self-Assembly in Poly(Ionic Liquid) Nanoparticles

Zhang, W., Kochovski, Z., Lu, Y., Schmidt, B. V. K. J., Antonietti, M., & Yuan, J. (2016). Internal Morphology-Controllable Self-Assembly in Poly(Ionic Liquid) Nanoparticles. ACS Nano, 10(8), 7731-7737. doi:10.1021/acsnano.6b03135.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-29C8-4 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-556E-B
Genre: Journal Article
Alternative Title : ACS Nano

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 Creators:
Zhang, Weiyi1, Author              
Kochovski, Zdravko, Author
Lu, Yan, Author
Schmidt, Bernhard V. K. J.2, Author              
Antonietti, Markus3, Author              
Yuan, Jiayin1, Author              
Affiliations:
1Jiayin Yuan, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863318              
2Bernhard Schmidt, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2149676              
3Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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 Abstract: Precise control of the interior and outer shapes of polymer nanoparticles has found broad interest in nanosciences, for example, in fundamental studies of their physical properties, colloidal behavior, and corresponding applications. Realizing such control below the 50 nm scale (i.e., a size scale close to individual polymer chains) requires accurate manipulation of polymerization techniques and a judicious choice of the chemical structure in monomers and/or polymers. Here, we constructed a series of well-defined sub-50 nm homopolymer nanoparticles with controllable shape and highly ordered, complex internal structures with sub-5 nm domain spacings, starting from 1-vinyl-1,2,4-triazolium-type ionic liquids in a one-pot dispersion polymerization. With cryogenic electron microscopy and tomography, a morphological evolution of particle shape and interior at this extremely small size end, unusual for polymer colloids, was identified and investigated in detail.

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 Dates: 2016-08-082016-08-23
 Publication Status: Published in print
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 Identifiers: DOI: 10.1021/acsnano.6b03135
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Title: ACS Nano
Source Genre: Journal
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Publ. Info: Washington, DC : American Chemical Society
Pages: - Volume / Issue: 10 (8) Sequence Number: - Start / End Page: 7731 - 7737 Identifier: ISSN: 1936-0851