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  Correlated Dynamics of the Motion of Proton-Hole Wave Packets in a Photoionized Water Cluster

Li, Z., Madjet, M.-E.-A., Vendrell, O., & Santra, R. (2013). Correlated Dynamics of the Motion of Proton-Hole Wave Packets in a Photoionized Water Cluster. Physical Review Letters, 110(3): 038302. doi:10.1103/PhysRevLett.110.038302.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-2309-F Version Permalink: http://hdl.handle.net/21.11116/0000-0003-5897-0
Genre: Journal Article

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PhysRevLett.110.038302.pdf (Publisher version), 2MB
 
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 Creators:
Li, Zheng1, 2, 3, Author              
Madjet, Mohamed El-Amine2, Author
Vendrell, Oriol2, Author
Santra, Robin2, 3, Author
Affiliations:
1International Max Planck Research School for Ultrafast Imaging & Structural Dynamics (IMPRS-UFAST), Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266714              
2Center for Free-Electron Laser Science, DESY, Notkestrasse 85, D-22607 Hamburg, Germany, ou_persistent22              
3Department of Physics, University of Hamburg, D-20355 Hamburg, Germany, ou_persistent22              

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Free keywords: PACS numbers: 82.20.Gk, 31.50.Gh, 33.80.Eh, 82.33.Fg
 Abstract: We explore the correlated dynamics of an electron hole and a proton after ionization of a protonated water cluster by extreme ultraviolet light. An ultrafast decay mechanism is found in which the proton-hole dynamics after the ionization are driven by electrostatic repulsion and involve a strong coupling between the nuclear and electronic degrees of freedom. We describe the system by a quantum-dynamical approach and show that nonadiabatic effects are a key element of the mechanism by which electron and proton repel each other and become localized at opposite sides of the cluster. Based on the generality of the decay mechanism, similar effects may be expected for other ionized systems featuring hydrogen bonds.

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Language(s): eng - English
 Dates: 2012-09-032013-01-152013-01-18
 Publication Status: Published in print
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.110.038302
arXiv: 1212.4686
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 110 (3) Sequence Number: 038302 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: /journals/resource/954925433406_1