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  Poly(ionic liquid)-Mediated Morphogenesis of Bismuth Sulfide with a Tunable Band Gap and Enhanced Electrocatalytic Properties

Gao, M.-R., Yu, S.-H., Yuan, J., Zhang, W., & Antonietti, M. (2016). Poly(ionic liquid)-Mediated Morphogenesis of Bismuth Sulfide with a Tunable Band Gap and Enhanced Electrocatalytic Properties. Angewandte Chemie, 128(41), 13004-13008. doi:10.1002/ange.201607221.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-603B-F Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-BA36-5
Genre: Journal Article

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 Creators:
Gao, Min-Rui1, Author
Yu, Shu-Hong, Author
Yuan, Jiayin1, Author              
Zhang, Weiyi1, Author              
Antonietti, Markus2, Author              
Affiliations:
1Jiayin Yuan, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863318              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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Free keywords: Anorganische Kristalle, Bismutsulfid, Morphogenese, Polymere ionische Flüssigkeiten, Polymerkontrollierte Kristallisation
 Abstract: Conventional polymer additives have a substantial impact on synthetic inorganic chemistry, but critical shortcomings remain; for example, low solubility in organic solvents and potential thermodynamic aggregates. Poly(ionic liquid)s have now been used as efficient additives that enable a high level control of bismuth sulfide crystals with significant size and morphological diversities. The bismuth sulfides exhibit tunable band structure as a result of the quantum size effects. Moreover, poly(ionic liquid)s are able to couple with as-synthesized bismuth sulfides chemically and endow a modified surface electronic structure, which allows resultant products to possess outstanding electrocatalytic performance for water oxidation, although its commercial counterpart is catalytically inert.

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 Dates: 2016-09-152016-10-04
 Publication Status: Published in print
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 Identifiers: DOI: 10.1002/ange.201607221
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Title: Angewandte Chemie
  Abbreviation : Angew. Chem.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 128 (41) Sequence Number: - Start / End Page: 13004 - 13008 Identifier: ISSN: 0044-8249