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  Disclosing the high activity of ceramic metallics in the oxygen evolution reaction : nickel materials as a case study

Ledendecker, M., Yang, X., Antonietti, M., & Shalom, M. (2016). Disclosing the high activity of ceramic metallics in the oxygen evolution reaction: nickel materials as a case study. ChemSusChem, 9(20), 2928-2932. doi:10.1002/cssc.201601128.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002B-78AF-E Version Permalink: https://hdl.handle.net/21.11116/0000-0007-E652-9
Genre: Journal Article

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 Creators:
Ledendecker, Marc1, Author           
Yang, Xiaofei, Author
Antonietti, Markus2, Author           
Shalom, Menny3, Author           
Affiliations:
1Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              
3Menny Shalom, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2205635              

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Free keywords: ceramic metallics, electrocatalysis, metallic alloys, oxygen evolution reaction, water splitting
 Abstract: Here, we elucidate the activity origin of ceramic nickel electrocatalysts in the oxygen evolution reaction (OER), ranging from nitrides, sulfides, and phosphides, as a case study that may be projected on almost any ceramic metallic. Our results show that regardless of the starting material, the formation of an active (oxy)hydroxide layer, acting as the real electrocatalyst during the OER, is unavoidable. Nevertheless, the in situ transformation into highly active (oxy)hydroxides leads to the formation of active catalysts for various applications.

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 Dates: 2016-09-212016
 Publication Status: Issued
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 Identifiers: DOI: 10.1002/cssc.201601128
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Title: ChemSusChem
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 9 (20) Sequence Number: - Start / End Page: 2928 - 2932 Identifier: ISSN: 1864-5631