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  Self-Organized Stationary Patterns in Networks of Bistable Chemical Reactions

Kouvaris, N. E., Sebek, M., Mikhailov, A. S., & Kiss, I. Z. (2016). Self-Organized Stationary Patterns in Networks of Bistable Chemical Reactions. Angewandte Chemie, 128(42), 13461-13465. doi:10.1002/ange.201607030.

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1609.07783.pdf (Preprint), 411KB
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 Creators:
Kouvaris, N. E.1, Author
Sebek, M.2, Author
Mikhailov, Alexander S.3, Author           
Kiss, I. Z.2, Author
Affiliations:
1Department of Physics, University of Barcelona, Martí i Franqùes 1, 08028 Barcelona (Spain), ou_persistent22              
2Department of Chemistry, Saint Louis University, 3501 Laclede Avenue, St. Louis, Missouri 63103 (USA), ou_persistent22              
3Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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 Abstract: Experiments with networks of discrete reactive bistable electrochemical elements organized in regular and nonregular tree networks are presented to confirm an alternative to the Turing mechanism for the formation of self-organized stationary patterns. The results show that the pattern formation can be described by the identification of domains that can be activated individually or in combinations. The method also enabled the localization of chemical reactions to network substructures and the identification of critical sites whose activation results in complete activation of the system. Although the experiments were performed with a specific nickel electrodissolution system, they reproduced all the salient dynamic behavior of a general network model with a single nonlinearity parameter. Thus, the considered pattern-formation mechanism is very robust, and similar behavior can be expected in other natural or engineered networked systems that exhibit, at least locally, a treelike structure.

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 Dates: 2016-07-202016-09-212016-10-10
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/ange.201607030
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Title: Angewandte Chemie
  Abbreviation : Angew. Chem.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: 4 Volume / Issue: 128 (42) Sequence Number: - Start / End Page: 13461 - 13465 Identifier: ISSN: 0044-8249
CoNE: https://pure.mpg.de/cone/journals/resource/954926979058_1