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  Anisotropic Self-Assembly of Organic–Inorganic Hybrid Microtoroids

Al-Rehili, S., Fhayli, K., Hammami, M. A., Moosa, B., Patil, S., Zhang, D., et al. (2016). Anisotropic Self-Assembly of Organic–Inorganic Hybrid Microtoroids. Journal of the American Chemical Society. doi:10.1021/jacs.6b10080.

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Datensatz-Permalink: https://hdl.handle.net/11858/00-001M-0000-002B-BCB2-E Versions-Permalink: https://hdl.handle.net/11858/00-001M-0000-002B-BCB3-C
Genre: Zeitschriftenartikel
Alternativer Titel : Journal of the American Chemical Society

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 Urheber:
Al-Rehili, Safa’a, Autor
Fhayli, Karim, Autor
Hammami, Mohamed Amen, Autor
Moosa, Basem, Autor
Patil, Sachin, Autor
Zhang, Daliang, Autor
Alharbi, Ohoud, Autor
Hedhili, Mohamed Nejib, Autor
Möhwald, Helmuth1, Autor           
Khashab, Niveen M., Autor
Affiliations:
1Helmuth Möhwald, Grenzflächen, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863312              

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 Zusammenfassung: Toroidal structures based on self-assembly of predesigned building blocks are well-established in the literature, but spontaneous self-organization to prepare such structures has not been reported to date. Here, organic–inorganic hybrid microtoroids synthesized by simultaneous coordination-driven assembly of amphiphilic molecules and hydrophilic polymers are reported. Mixing amphiphilic molecules with iron(III) chloride and hydrophilic polymers in water leads, within minutes, to the formation of starlike nanostructures. A spontaneous self-organization of these nanostructures is then triggered to form stable hybrid microtoroids. Interestingly, the toroids exhibit anisotropic hierarchical growth, giving rise to a layered toroidal framework. These microstructures are mechanically robust and can act as templates to host metallic nanoparticles such as gold and silver. Understanding the nature of spontaneous assembly driven by coordination multiple non-covalent interactions can help explain the well-ordered complexity of many biological organisms in addition to expanding the available tools to mimic such structures at a molecular level.

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 Datum: 2016-10-24
 Publikationsstatus: Online veröffentlicht
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 Ort, Verlag, Ausgabe: -
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 Art der Begutachtung: -
 Identifikatoren: DOI: 10.1021/jacs.6b10080
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Titel: Journal of the American Chemical Society
  Andere : J. Am. Chem. Soc.
  Kurztitel : JACS
Genre der Quelle: Zeitschrift
 Urheber:
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Ort, Verlag, Ausgabe: Washington, DC : American Chemical Society
Seiten: - Band / Heft: - Artikelnummer: - Start- / Endseite: - Identifikator: ISSN: 0002-7863