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  Long-Range Domain Structure and Symmetry Engineering by Interfacial Oxygen Octahedral Coupling at Heterostructure Interface

Liao, Z., Green, R. J., Gauquelin, N., Macke, S., Li, L., Gonnissen, J., et al. (2016). Long-Range Domain Structure and Symmetry Engineering by Interfacial Oxygen Octahedral Coupling at Heterostructure Interface. Advanced Functional Materials, 26(36), 6627-6634. doi:10.1002/adfm.201602155.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002B-B98E-B Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002E-1A4F-4
Genre: Journal Article

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 Creators:
Liao, Zhaoliang1, Author
Green, Robert J.2, Author              
Gauquelin, Nicolas1, Author
Macke, Sebastian1, Author
Li, Lin1, Author
Gonnissen, Julie1, Author
Sutarto, Ronny1, Author
Houwman, Evert P.1, Author
Zhong, Zhicheng1, Author
Van Aert, Sandra1, Author
Verbeeck, Johan1, Author
Sawatzky, George A.1, Author
Huijben, Mark1, Author
Koster, Gertjan1, Author
Rijnders, Guus1, Author
Affiliations:
1External Organizations, ou_persistent22              
2Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863445              

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 Abstract: In epitaxial thin film systems, the crystal structure and its symmetry deviate from the bulk counterpart due to various mechanisms such as epitaxial strain and interfacial structural coupling, which is accompanyed by a change in their properties. In perovskite materials, the crystal symmetry can be described by rotations of sixfold coordinated transition metal oxygen octahedra, which are found to be altered at interfaces. Here, it is unraveled how the local oxygen octahedral coupling at perovskite heterostructural interfaces strongly influences the domain structure and symmetry of the epitaxial films resulting in design rules to induce various structures in thin films using carefully selected combinations of substrate/buffer/film. Very interestingly it is discovered that these combinations lead to structure changes throughout the full thickness of the film. The results provide a deep insight into understanding the origin of induced structures in a perovskite heterostructure and an intelligent route to achieve unique functional properties.

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Language(s): eng - English
 Dates: 2016-06-222016-06-22
 Publication Status: Published in print
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: -
 Identifiers: ISI: 000384809800010
DOI: 10.1002/adfm.201602155
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Title: Advanced Functional Materials
  Other : Adv. Funct. Mater.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH Verlag GmbH
Pages: - Volume / Issue: 26 (36) Sequence Number: - Start / End Page: 6627 - 6634 Identifier: ISSN: 1616-301X
CoNE: /journals/resource/954925596563