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  Hetero-site-specific X-ray pump-probe spectroscopy for femtosecond intramolecular dynamics.

Picón, A., Lehmann, C. S., Bostedt, C., Rudenko, A., Marinelli, A., Osipov, T., et al. (2016). Hetero-site-specific X-ray pump-probe spectroscopy for femtosecond intramolecular dynamics. Nature Communications, 7: 11652. doi:10.1038/ncomms11652.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002C-0D41-5 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002C-896E-A
Genre: Journal Article

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 Creators:
Picón, A., Author
Lehmann, C. S., Author
Bostedt, C., Author
Rudenko, A., Author
Marinelli, A., Author
Osipov, T., Author
Rolles, D.1, Author              
Berrah, N., Author
Bomme, C.1, Author              
Bucher, M., Author
Doumy, G., Author
Erk, B., Author
Ferguson, K. R., Author
Gorkhover, T., Author
Ho, P. J., Author
Kanter, E. P., Author
Krässig, B., Author
Krzywinski, J., Author
Lutman, A. A., Author
March, A. M., Author
Moonshiram, D., AuthorRay, D., AuthorYoung, L., AuthorPratt, S. T., AuthorSouthworth, S. H., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society, ou_578564              

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 Abstract: New capabilities at X-ray free-electron laser facilities allow the generation of two-colour femtosecond X-ray pulses, opening the possibility of performing ultrafast studies of X-ray-induced phenomena. Particularly, the experimental realization of hetero-site-specific X-ray-pump/X-ray-probe spectroscopy is of special interest, in which an X-ray pump pulse is absorbed at one site within a molecule and an X-ray probe pulse follows the X-ray-induced dynamics at another site within the same molecule. Here we show experimental evidence of a hetero-site pump-probe signal. By using two-colour 10-fs X-ray pulses, we are able to observe the femtosecond time dependence for the formation of F ions during the fragmentation of XeF2 molecules following X-ray absorption at the Xe site.

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Language(s): eng - English
 Dates: 2016-05-23
 Publication Status: Published online
 Pages: -
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 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1038/ncomms11652
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Title: Nature Communications
Source Genre: Journal
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Pages: 6 Volume / Issue: 7 Sequence Number: 11652 Start / End Page: - Identifier: -