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  Sensing the wavefront of x-ray free-electron lasers using aerosol spheres.

Loh, N. D., Starodub, D., Lomb, L., Hampton, C. Y., Martin, A. V., Sierra, R. G., et al. (2013). Sensing the wavefront of x-ray free-electron lasers using aerosol spheres. Optics Express, 21(10), 12385-12394. doi:10.1364/OE.21.012385.

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Loh, N. D., Author
Starodub, D., Author
Lomb, L., Author
Hampton, C. Y., Author
Martin, A. V., Author
Sierra, R. G., Author
Barty, A., Author
Aquila, A., Author
Schulz, J., Author
Steinbrener, J., Author
Shoeman, R. L., Author
Kassemeyer, S., Author
Bostedt, Christoph, Author
Bozek, J., Author
Epp, S. W., Author
Erk, B., Author
Hartmann, R., Author
Rolles, D.1, Author              
Rudenko, A., Author
Rudek, B., Author
Foucar, L., AuthorKimmel, N., AuthorWeidenspointner, G., AuthorHauser, G., AuthorHoll, P., AuthorPedersoli, E., AuthorLiang, M., AuthorHunter, M. S., AuthorGumprecht, L., AuthorCoppola, N., AuthorWunderer, C., AuthorGraafsma, H., AuthorMaia, F. R.N.C., AuthorEkeberg, T., AuthorHantke, M., AuthorFleckenstein, H., AuthorHirsemann, H., AuthorNass, K., AuthorWhite, T. A., AuthorTobias, H. J., AuthorFarquar, G. R., AuthorBenner, W. H., AuthorHau-Riege, S., AuthorReich, C., AuthorHartmann, A., AuthorSoltau, H., AuthorMarchesini, S., AuthorBajt, S., AuthorBarthelmess, M., AuthorStrueder, L., AuthorUllrich, J., AuthorBucksbaum, P., AuthorFrank, M., AuthorSchlichting, I., AuthorChapman, H. N., AuthorBogan, M. J., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society, ou_578564              

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 Abstract: Characterizing intense, focused x-ray free electron laser (FEL) pulses is crucial for their use in diffractive imaging. We describe how the distribution of average phase tilts and intensities on hard x-ray pulses with peak intensities of 1021 W/m2 can be retrieved from an ensemble of diffraction patterns produced by 70 nm-radius polystyrene spheres, in a manner that mimics wavefront sensors. Besides showing that an adaptive geometric correction may be necessary for diffraction data from randomly injected sample sources, our paper demonstrates the possibility of collecting statistics on structured pulses using only the diffraction patterns they generate and highlights the imperative to study its impact on single-particle diffractive imaging.

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Language(s): eng - English
 Dates: 2013-05-132013-05-20
 Publication Status: Published in print
 Pages: -
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 Rev. Type: Peer
 Identifiers: DOI: 10.1364/OE.21.012385
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Title: Optics Express
Source Genre: Journal
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Pages: - Volume / Issue: 21 (10) Sequence Number: - Start / End Page: 12385 - 12394 Identifier: -