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  Study of iron-catalysed growth of beta-Ga2O3 nanowires and their detailed characterization using TEM, Raman and cathodoluminescence techniques

Kumar, S., Sarau, G., Tessarek, C., Bashouti, M. Y., Haehnel, A., Christiansen, S., et al. (2014). Study of iron-catalysed growth of beta-Ga2O3 nanowires and their detailed characterization using TEM, Raman and cathodoluminescence techniques. JOURNAL OF PHYSICS D-APPLIED PHYSICS, 47(43): 435101. doi:10.1088/0022-3727/47/43/435101.

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 Creators:
Kumar, Sudheer1, Author
Sarau, G.2, Author              
Tessarek, C.2, Author              
Bashouti, Muhammad Y.2, Author              
Haehnel, A.1, Author
Christiansen, S.2, 3, Author              
Singh, R.1, Author
Affiliations:
1external, ou_persistent22              
2Micro- & Nanostructuring, Technology Development and Service Units, Max Planck Institute for the Science of Light, Max Planck Society, ou_2364725              
3Christiansen Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society, ou_2364716              

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Free keywords: GALLIUM OXIDE NANOWIRES; GA2O3 NANOWIRES; ORGANOMETALLIC PRECURSOR; OPTICAL-PROPERTIES; CVD TECHNIQUE; GAS SENSORS; THIN-FILMS; SINGLE; PHOTOLUMINESCENCE; LUMINESCENCEPhysics; gallium oxide nanowires; Raman spectra; cathodoluminescence; scanning transmission electron microscopy; chemical vapour deposition;
 Abstract: In this paper, we demonstrate a new catalyst (Fe) to grow single crystalline beta-gallium oxide (beta-Ga2O3) nanowires (NWs) via the vapour-liquid-solid mechanism using the chemical vapour deposition technique. The structural studies of these NWs showed the highly crystalline monoclinic phase of Ga2O3. This was confirmed by detailed scanning transmission electron microscope investigations demonstrating the NW to be single crystalline beta-Ga2O3, growing along the normal of the (1 (1) over bar (1) over bar) plane. We also compared Raman and cathodoluminescence (CL) properties of the as-grown beta-Ga2O3 NWs with a bulk Ga2O3 single crystal grown by the Czochralski method. It was observed that Raman peak positions of a single beta-Ga2O3 NW had a red frequency shift of about 0.3-1.4 cm(-1) as compared to a bulk Ga2O3 single crystal, which was in fact quite small. In addition, the CL measurements of beta-Ga2O3 NWs and the bulk Ga2O3 single crystal exhibited similar spectra, having a strong broad UV-blue emission band and a weak red emission band. Moreover, the structural, morphological and optical properties of Fe-catalysed beta-Ga2O3 NWs were comparable to those of Au-catalysed beta-Ga2O3 NWs.

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Language(s): eng - English
 Dates: 2014
 Publication Status: Published online
 Pages: 10
 Publishing info: -
 Table of Contents: -
 Rev. Type: -
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Title: JOURNAL OF PHYSICS D-APPLIED PHYSICS
Source Genre: Journal
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Publ. Info: TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND : IOP PUBLISHING LTD
Pages: - Volume / Issue: 47 (43) Sequence Number: 435101 Start / End Page: - Identifier: ISSN: 0022-3727