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  Single-Photon Spectroscopy of a Single Molecule

Rezus, Y. L. A., Walt, S. G., Lettow, R., Renn, A., Zumofen, G., Goetzinger, S., et al. (2012). Single-Photon Spectroscopy of a Single Molecule. Physical Review Letters, 108: 093601. doi:10.1103/PhysRevLett.108.093601.

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 Creators:
Rezus, Y. L. A.1, Author
Walt, S. G.1, Author
Lettow, R.1, Author
Renn, A.1, Author
Zumofen, G.1, Author
Goetzinger, S.2, Author           
Sandoghdar, V.2, Author           
Affiliations:
1external, ou_persistent22              
2Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society, ou_2364722              

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Free keywords: EMISSION; FLUORESCENCE; TRANSISTOR; EXTINCTION; PLASMONSPhysics;
 Abstract: Efficient interaction of light and matter at the ultimate limit of single photons and single emitters is of great interest from a fundamental point of view and for emerging applications in quantum engineering. However, the difficulty of generating single-photon streams with specific wavelengths, bandwidths, and power as well as the weak interaction probability of a single photon with an optical emitter pose a formidable challenge toward this goal. Here, we demonstrate a general approach based on the creation of single photons from a single emitter and their use for performing spectroscopy on a second emitter situated at a distance. While this first proof of principle realization uses organic molecules as emitters, the scheme is readily extendable to quantum dots and color centers. Our work ushers in a new line of experiments that provide access to the coherent and nonlinear couplings of few emitters and few propagating photons.

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Language(s): eng - English
 Dates: 2012
 Publication Status: Published online
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: -
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 108 Sequence Number: 093601 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1