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  Self-assembled carbon nitride for photocatalytic hydrogen evolution and degradation of p-nitrophenol

Sun, J., Xu, J., Grafmüller, A., Huang, X., Liedel, C., Algara-Siller, G., et al. (2017). Self-assembled carbon nitride for photocatalytic hydrogen evolution and degradation of p-nitrophenol. Applied Catalysis B: Environmental, 205, 1-10. doi:10.1016/j.apcatb.2016.12.030.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002C-218F-B Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-C03E-5
Genre: Journal Article

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 Creators:
Sun, Jingwen1, Author
Xu, Jingsan1, Author              
Grafmüller, Andrea2, Author              
Huang, Xing, Author
Liedel, Clemens3, Author              
Algara-Siller, Gerardo, Author
Willinger, Marc4, Author
Yang, Can, Author
Fu, Yongsheng, Author
Wang, Xin, Author
Shalom, Menny1, Author              
Affiliations:
1Menny Shalom, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2205635              
2Andrea Grafmüller, Theorie & Bio-Systeme, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863323              
3Clemens Liedel, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2288694              
4Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              

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Free keywords: Carbon nitride; Sequential solvent treatment; H2 evolution; Photodegradation
 Abstract: Carbon nitride has attracted significant interest as robust, low-cost alternative to metal-based materials in fields such as photo, electro and heterogeneous catalysis. However, the properties of the final material are hard to control by traditional synthetic methods Herein, we introduce a new strategy of material design that allows controlling the desired properties of the final material already from the molecular level by sequential solvent treatment of supramolecular aggregates that serve as the reactants. Due to in situ formation of a thermodynamic driven energy levels gradient, the as-prepared carbon nitride exhibits almost 10 times higher activity than the traditional carbon nitride (calcined from melamine) in the hydrogen evolution text. As a multifunctional catalyst, the core-shell like carbon nitride also shows a superior catalytic degradation activity for RhB and p-nitrophenol.

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 Dates: 2016-12-092017-05-15
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Method: -
 Identifiers: DOI: 10.1016/j.apcatb.2016.12.030
BibTex Citekey: Sun2016
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Title: Applied Catalysis B: Environmental
Source Genre: Journal
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Publ. Info: Amsterdam : Elsevier
Pages: - Volume / Issue: 205 Sequence Number: - Start / End Page: 1 - 10 Identifier: ISSN: 0926-3373