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  Imaging the He2 quantum halo state using a free electron laser

Zeller, S., Kunitski, M., Voigtsberger, J., Kalinin, A., Schottelius, A., Schober, C., et al. (2016). Imaging the He2 quantum halo state using a free electron laser. Proceedings of the National Academy of Sciences of the USA, 113(51), 14651-14655. doi:10.1073/pnas.1610688113.

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Zeller, Stefan1, Author
Kunitski, Maksim1, Author
Voigtsberger, Jörg1, Author
Kalinin, Anton1, Author
Schottelius, Alexander1, Author
Schober, Carl1, Author
Waitz, Markus1, Author
Sann, Hendrik1, Author
Hartung, Alexander1, Author
Bauer, Tobias1, Author
Pitzer, Martin1, Author
Trinter, Florian1, Author
Goihl, Christoph1, Author
Janke, Christian1, Author
Richter, Martin1, Author
Kastirke, Gregor1, Author
Weller, Miriam1, Author
Czasch, Achim1, Author
Kitzler, Markus2, Author
Braune, Markus3, Author
Grisenti, Robert E.1, 4, AuthorSchöllkopf, Wieland5, Author           Schmidt, Lothar Ph. H.1, AuthorSchöffler, Markus S.1, AuthorWilliams, Joshua B.6, AuthorJahnke, Till1, AuthorDörner, Reinhard1, Author more..
Affiliations:
1Institut für Kernphysik, Goethe-Universität Frankfurt, 60438 Frankfurt, Germany, ou_persistent22              
2Photonics Institute, Vienna University of Technology, 1040 Vienna, Austria, ou_persistent22              
3Deutsches Elektronen-Synchrotron, 22607 Hamburg, Germany, ou_persistent22              
4GSI Helmholtz Centre for Heavy Ion Research, 64291 Darmstadt, Germany, ou_persistent22              
5Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
6Department of Physics, University of Nevada, Reno, NV 89557, ou_persistent22              

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 Abstract: Quantum tunneling is a ubiquitous phenomenon in nature and crucial for many technological applications. It allows quantum particles to reach regions in space which are energetically not accessible according to classical mechanics. In this “tunneling region,” the particle density is known to decay exponentially. This behavior is universal across all energy scales from nuclear physics to chemistry and solid state systems. Although typically only a small fraction of a particle wavefunction extends into the tunneling region, we present here an extreme quantum system: a gigantic molecule consisting of two helium atoms, with an 80% probability that its two nuclei will be found in this classical forbidden region. This circumstance allows us to directly image the exponentially decaying density of a tunneling particle, which we achieved for over two orders of magnitude. Imaging a tunneling particle shows one of the few features of our world that is truly universal: the probability to find one of the constituents of bound matter far away is never zero but decreases exponentially. The results were obtained by Coulomb explosion imaging using a free electron laser and furthermore yielded He2’s binding energy of 151.9±13.3 neV, which is in agreement with most recent calculations.

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 Dates: 2016-06-302016-11-032016-12-062016-12-20
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1073/pnas.1610688113
 Degree: -

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Title: Proceedings of the National Academy of Sciences of the USA
  Abbreviation : PNAS
Source Genre: Journal
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Publ. Info: Washington, D.C. : National Academy of Sciences
Pages: 5 Volume / Issue: 113 (51) Sequence Number: - Start / End Page: 14651 - 14655 Identifier: ISSN: 0027-8424
CoNE: https://pure.mpg.de/cone/journals/resource/954925427230