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  Lignin-based polymeric surfactants for emulsion polymerization

Schmidt, B. V. K. J., Molinari, V., Esposito, D., Tauer, K., & Antonietti, M. (2017). Lignin-based polymeric surfactants for emulsion polymerization. Polymer, 112, 418-426. doi:10.1016/j.polymer.2017.02.036.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002C-6254-B Version Permalink: https://hdl.handle.net/21.11116/0000-0007-F32C-6
Genre: Journal Article

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 Creators:
Schmidt, Bernhard V. K. J.1, Author           
Molinari, Valerio2, Author           
Esposito, Davide2, Author           
Tauer, Klaus3, Author           
Antonietti, Markus4, Author           
Affiliations:
1Bernhard Schmidt, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2149676              
2Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863315              
3Klaus Tauer, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863320              
4Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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 Abstract: A non-ionic surfactant system is synthesized by standard grafting of poly (ethylene oxide) from renewable lignin fragments and used for the emulsion polymerization of styrene. The lignin precursors is formed by hydrogenolysis and utilized as initiator for the oxyanionic polymerization of ethylene oxide leading to amphiphilic polymers, very similar to standard nonionic surfactant synthesis. Subsequently, the formed amphiphilic polymers are employed as stabilizers in the heterophase polymerization of styrene with various initiators. Poly (styrene) latexes with solids contents of up to 21% depending on stabilizer concentration have been obtained. Stabilizer efficiencies and performances were nicely comparable with those of nonylphenol-based, non-ionic industrial performance surfactants.

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 Dates: 2017-02-102017
 Publication Status: Issued
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 Identifiers: DOI: 10.1016/j.polymer.2017.02.036
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Title: Polymer
  Other : Polymer
Source Genre: Journal
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Publ. Info: Guildford, England : Elsevier
Pages: - Volume / Issue: 112 Sequence Number: - Start / End Page: 418 - 426 Identifier: ISSN: 0032-3861