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  Order-disorder transition in surface-induced nanopattern of diblock copolymer films

Spatz, J. P., Eibeck, P., Mössmer, S., Möller, M., Kramarenko, E. Y., Khalatur, P. G., et al. (2000). Order-disorder transition in surface-induced nanopattern of diblock copolymer films. Macromolecules, 33(1), 150-157. doi:10.1021/ma990751p.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002A-14C6-2 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-002E-7D8D-C
Genre: Journal Article

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Makromol_33_2000_150.pdf (Any fulltext), 391KB
 
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http://pubs.acs.org/doi/pdf/10.1021/ma990751p (Any fulltext)
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https://dx.doi.org/10.1021/ma990751p (Any fulltext)
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 Creators:
Spatz, Joachim P.1, 2, Author           
Eibeck, Peter, Author
Mössmer, Stefan, Author
Möller, Martin, Author
Kramarenko, Elena Yu., Author
Khalatur, Pavel. G., Author
Potemkin, Igor I., Author
Khokhlov, Alexei R., Author
Winkler, Roland G., Author
Reineker, Peter, Author
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              
2Biophysical Chemistry, Institute of Physical Chemistry, University of Heidelberg, 69120 Heidelberg, Germany, ou_persistent22              

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 Abstract: Formation of surface-induced nanopattern (SINPAT) in ultrathin diblock copolymer films is studied by scanning force microscopy and Monte Carlo simulation. The pattern is caused by strong adsorption of one of the two blocks forming a quasi-two-dimensional coil while the other block dewets this adsorption layer. Scanning force microscopy allowed to observe an order−disorder transition for a SINPAT film of polystyrene-block-poly(2-vinylpyridine) on mica when the length of the dewetting polystyrene block was varied. The experimental data are compared with the Monte Carlo simulations which demonstrate how the pattern formation depends on the degree of polymerization of the dewetting block and the unfavorable interaction potential between the different components.

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Language(s): eng - English
 Dates: 1999-05-141999-12-102000
 Publication Status: Issued
 Pages: 8
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 Table of Contents: -
 Rev. Type: -
 Identifiers: ISI: ISI:000084799300026
ISSN: 0024-9297
DOI: 10.1021/ma990751p
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Title: Macromolecules
Source Genre: Journal
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Publ. Info: Washington, D.C. : American Chemical Society
Pages: - Volume / Issue: 33 (1) Sequence Number: - Start / End Page: 150 - 157 Identifier: ISSN: 0024-9297
CoNE: https://pure.mpg.de/cone/journals/resource/954925421108