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  Efficiency of Ni nanoparticles supported on hierarchical porous nitrogen-doped carbon for hydrogenolysis of Kraft lignin in flow and batch systems

Lama, S., Pampel, J., Fellinger, T.-P., Beškoski, V. P., Slavković-Beškoski, L., Antonietti, M., et al. (2017). Efficiency of Ni nanoparticles supported on hierarchical porous nitrogen-doped carbon for hydrogenolysis of Kraft lignin in flow and batch systems. ACS Sustainable Chemistry & Engineering, 5(3), 2415-2420. doi:10.1021/acssuschemeng.6b02761.

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Lama, Sandy1, Autor           
Pampel, Jonas2, Autor           
Fellinger, Tim-Patrick2, Autor           
Beškoski, Vladimir P., Autor
Slavković-Beškoski, Latinka, Autor
Antonietti, Markus3, Autor           
Molinari, Valerio4, 5, Autor           
Affiliations:
1Martin Oschatz, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2364733              
2Tim Fellinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863322              
3Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              
4Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863315              
5Valerio Molinari, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2385693              

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 Zusammenfassung: Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni–C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.

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 Datum: 2017
 Publikationsstatus: Erschienen
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 Identifikatoren: DOI: 10.1021/acssuschemeng.6b02761
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Titel: ACS Sustainable Chemistry & Engineering
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Washington, DC : American Chemical Society
Seiten: - Band / Heft: 5 (3) Artikelnummer: - Start- / Endseite: 2415 - 2420 Identifikator: ISSN: 2168-0485