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  Pd@ionosilica as heterogeneous hydrogenation catalyst for continuous flow reductive upgrade of cinnamaldehyde

Braun, M., Thach, U. D., Prelot, B., Hesemann, P., & Esposito, D. (2017). Pd@ionosilica as heterogeneous hydrogenation catalyst for continuous flow reductive upgrade of cinnamaldehyde. Journal of Chemical Technology & Biotechnology, 92(9), 2229-2235. doi:10.1002/jctb.5278.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-2D2A-E Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002E-9643-A
Genre: Journal Article

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 Creators:
Braun, Max1, Author              
Thach, Ut Dong, Author
Prelot, Bénédicte, Author
Hesemann, Peter, Author
Esposito, Davide1, Author              
Affiliations:
1Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863315              

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Free keywords: ionosilica, palladium nanoparticles, biomass, reduction, hydrogenation
 Abstract: BACKGROUND: The effective exploitation of biomass for the preparation of fuels and platform chemicals requires the development of novel catalysts and catalytic methods. In this regard, ionosilicas appear as promising candidates due to their properties and tenability. RESULTS: A novel Pd@ionosilica is prepared by a straightforward ion exchange method based on amorphous ionosilica and sodium tetrachloropalladate. The resulting hybrid material is evaluated as catalyst for the continuous flow reduction of cinnamaldehyde as exemplary biorefinery case study. CONCLUSION: This work reports the application of metal@ionosilica hybrid materials as catalysts for the continuous flow upgrade of bio-sourced molecules, showing promising results in the case of cinnamaldehyde, here used as exemplary compound. The findings disclosed in this paper provide interesting insights for the development of second generation metal@ionosilica composites for catalytic applications within biorefinery.

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 Dates: 2017-03-142017-09
 Publication Status: Published in print
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 Identifiers: DOI: 10.1002/jctb.5278
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Title: Journal of Chemical Technology & Biotechnology
  Alternative Title : J. Chem. Technol. Biotechnol.
Source Genre: Journal
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Publ. Info: Hoboken, NJ : John Wiley & Sons
Pages: - Volume / Issue: 92 (9) Sequence Number: - Start / End Page: 2229 - 2235 Identifier: ISSN: 1097-4660