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  On the Bethe-Wigner-Shapiro limit of the rate coefficient for the capture of a rotating quadrupolar polarisable diatom by an ion.

Nikitin, E. E., & Troe, J. (2017). On the Bethe-Wigner-Shapiro limit of the rate coefficient for the capture of a rotating quadrupolar polarisable diatom by an ion. Molecular Physics, 115(4), 432-436. doi:10.1080/00268976.2016.1269964.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002C-E651-4 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002C-E654-D
Genre: Journal Article

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2418114.pdf (Publisher version), 608KB
 
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 Creators:
Nikitin, E. E.1, Author              
Troe, J.1, Author              
Affiliations:
1Emeritus Group of Spectroscopy and Photochemical Kinetics, MPI for Biophysical Chemistry, Max Planck Society, ou_578625              

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Free keywords: Low-temperature capture processes, Bethe–Shapiro–Wigner limit
 Abstract: The low-energy (Bethe–Wigner–Shapiro) behaviour of the rate coefficient for capture of a polarisable quadrupolar rotationally excited diatom by an ion is calculated. The multichannel character of capture shows itself in the dependence of the effective attractive potential on the intrinsic angular momentum of the diatom and in a nonadiabatic diagonal correction to the potential. The predicted energy dependence of the rate coefficients is compared with previous numerically accurate results for the capture of H2 molecules by H2+ ions.

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Language(s): eng - English
 Dates: 2016-12-222017
 Publication Status: Published in print
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 Rev. Method: Peer
 Identifiers: DOI: 10.1080/00268976.2016.1269964
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Title: Molecular Physics
Source Genre: Journal
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Pages: - Volume / Issue: 115 (4) Sequence Number: - Start / End Page: 432 - 436 Identifier: -