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  Jitter-correction for IR/UV-XUV pump-probe experiments at the FLASH free-electron laser.

Savelyev, E., Boll, R., Bomme, C., Schirmel, N., Redlin, H., Erk, B., et al. (2017). Jitter-correction for IR/UV-XUV pump-probe experiments at the FLASH free-electron laser. New Journal of Physics, 19: 043009. doi:10.1088/1367-2630/aa652d.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-3FB9-E Version Permalink: http://hdl.handle.net/21.11116/0000-0001-4B85-5
Genre: Journal Article

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 Creators:
Savelyev, E., Author
Boll, R., Author
Bomme, C., Author
Schirmel, N., Author
Redlin, H., Author
Erk, B., Author
Düsterer, S., Author
Müller, E., Author
Höppner, H., Author
Toleikis, S., Author
Müller, J., Author
Czwalinna, M. K., Author
Treusch, R., Author
Kierspel, T., Author
Mullins, T., Author
Trippel, S., Author
Wiese, J., Author
Küpper, J., Author
Brausse, F., Author
Krecinic, F., Author
Rouzee, A., AuthorRudawski, P., AuthorJohnsson, P., AuthorAmini, K., AuthorLauer, A., AuthorBurt, M., AuthorBrouard, M., AuthorChristensen, L., AuthorThogersen, J., AuthorStapelfeldt, H., AuthorBerrah, N., AuthorMüller, M., AuthorUlmer, A., AuthorTechert, S.1, Author              Rudenko, A., AuthorRolles, D., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for biophysical chemistry, Max Planck Society, ou_578564              

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Free keywords: free-electron laser; pump-probe experiments; photodissociation; velocity map imaging; time-resolved ion imaging
 Abstract: In pump-probe experiments employing a free-electron laser (FEL) in combination with a synchronized optical femtosecond laser, the arrival-time jitter between the FEL pulse and the optical laser pulse often severely limits the temporal resolution that can be achieved. Here, we present a pump-probe experiment on the UV-induced dissociation of 2,6-difluoroiodobenzene (C6H3F2I) molecules performed at the FLASH FEL that takes advantage of recent upgrades of the FLASH timing and synchronization system to obtain high-quality data that are not limited by the FEL arrival-time jitter. Wediscuss in detail the necessary data analysis steps and describe the origin of the timedependent effects in the yields and kinetic energies of the fragment ions that we observe in the experiment.

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Language(s): eng - English
 Dates: 2017-04-10
 Publication Status: Published online
 Pages: -
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 Rev. Method: Peer
 Identifiers: DOI: 10.1088/1367-2630/aa652d
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Title: New Journal of Physics
Source Genre: Journal
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Pages: 13 Volume / Issue: 19 Sequence Number: 043009 Start / End Page: - Identifier: -