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  Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera.

Amini, K., Boll, R., Lauer, A., Burt, M., Lee, J. W. L., Christensen, L., et al. (2017). Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera. The Journal of Chemical Physics, 147(1): 013933. doi:10.1063/1.4982220.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-6F29-6 Version Permalink: http://hdl.handle.net/21.11116/0000-0001-449F-0
Genre: Journal Article

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 Creators:
Amini, K., Author
Boll, R.1, Author              
Lauer, A., Author
Burt, M., Author
Lee, J. W. L., Author
Christensen, L., Author
Brausse, F., Author
Mullins, T., Author
Savelyev, E., Author
Ablikim, U., Author
Berrah, N., Author
Bomme, C., Author
Düsterer, S., Author
Erk, B., Author
Höppner, H., Author
Johnsson, P., Author
Kierspel, T., Author
Krecinic, F., Author
Küpper, J., Author
Müller, M., Author
Müller, E., AuthorRedlin, H., AuthorRouzee, A., AuthorSchirmel, N., AuthorThogersen, J., AuthorTechert, S.1, Author              Toleikis, S., AuthorTreusch, R., AuthorTrippel, S., AuthorUlmer, A., AuthorWiese, J., AuthorVallance, C., AuthorRudenko, A., AuthorStapelfeldt, H., AuthorBrouard, M., AuthorRolles, D., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society, ou_578564              

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 Abstract: Laser-induced adiabatic alignment and mixed-field orientation of 2,6-difluoroiodobenzene (C6H3F2I) molecules are probed by Coulomb explosion imaging following either near-infrared strong-field ionization or extreme-ultraviolet multi-photon inner-shell ionization using free-electron laser pulses. The resulting photoelectrons and fragment ions are captured by a double-sided velocity map imaging spectrometer and projected onto two position-sensitive detectors. The ion side of the spectrometer is equipped with a pixel imaging mass spectrometry camera, a time-stamping pixelated detector that can record the hit positions and arrival times of up to four ions per pixel per acquisition cycle. Thus, the time-of-flight trace and ion momentum distributions for all fragments can be recorded simultaneously. We show that we can obtain a high degree of one-and three-dimensional alignment and mixed-field orientation and compare the Coulomb explosion process induced at both wavelengths.

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Language(s): eng - English
 Dates: 2017-05-092017-07-07
 Publication Status: Published in print
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 Rev. Method: Peer
 Identifiers: DOI: 10.1063/1.4982220
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Title: The Journal of Chemical Physics
Source Genre: Journal
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Pages: 8 Volume / Issue: 147 (1) Sequence Number: 013933 Start / End Page: - Identifier: -