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  Sensitivities of Amazonian clouds to aerosols and updraft speed

Cecchini, M. A., Machado, L. A. T., Andreae, M. O., Martin, S. T., Albrecht, R. I., Artaxo, P., Barbosa, H. M. J., Borrmann, S., Fütterer, D., Jurkat, T., Mahnke, C., Minikin, A., Molleker, S., Pöhlker, M. L., Pöschl, U., Rosenfeld, D., Voigt, C., Weinzierl, B., & Wendisch, M. (2017). Sensitivities of Amazonian clouds to aerosols and updraft speed. Atmospheric Chemistry and Physics Discussions, 17.

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資料種別: 成果報告書

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 作成者:
Cecchini, Micael A., 著者
Machado, Luiz A. T., 著者
Andreae, M. O.1, 著者           
Martin, Scot T., 著者
Albrecht, Rachel I., 著者
Artaxo, Paulo, 著者
Barbosa, Henrique M. J., 著者
Borrmann, S.2, 著者           
Fütterer, Daniel, 著者
Jurkat, Tina, 著者
Mahnke, Christoph2, 著者           
Minikin, Andreas, 著者
Molleker, S.2, 著者           
Pöhlker, M. L.3, 著者           
Pöschl, U.3, 著者           
Rosenfeld, Daniel, 著者
Voigt, Christiane, 著者
Weinzierl, Bernadett, 著者
Wendisch, Manfred, 著者
所属:
1Biogeochemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826286              
2Particle Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826291              
3Multiphase Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826290              

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 要旨: The effects of aerosol particles and updraft speed on warm-phase cloud microphysical properties are studied in the Amazon region as part of the ACRIDICON-CHUVA experiment. Here we expand the sensitivity analysis usually found in the literature by concomitantly considering cloud evolution, putting the sensitivity quantifications into perspective in relation to in-cloud processing, and by considering the effects on droplet size distribution (DSD) shape. Our in-situ aircraft measurements over the Amazon basin cover a wide range of particle concentration and thermodynamic conditions, from the pristine regions over coastal and forested areas to the highly biomass-burning-polluted southern Amazon. The quantitative results show that particle concentration is the primary driver for the vertical profiles of effective diameter and droplet concentration in the warm phase of Amazonian convective clouds, while updraft speeds have a modulating role in the latter and in total condensed water. The cloud microphysical properties were found to be highly variable with altitude above cloud base, which we used as a proxy for cloud evolution since it is a measure of the time droplets were subject to cloud processing. We show that DSD shape is crucial in understanding cloud sensitivities. The aerosol effect on DSD shape was found to vary with altitude, which can help models to better constrain the indirect aerosol effect on climate.

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言語: eng - English
 日付: 2017
 出版の状態: 出版
 ページ: -
 出版情報: -
 目次: -
 査読: -
 識別子(DOI, ISBNなど): DOI: 10.5194/acp-2017-89
 学位: -

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出版物 1

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出版物名: Atmospheric Chemistry and Physics Discussions
  省略形 : Atmos. Chem. Phys. Discuss.
種別: 学術雑誌
 著者・編者:
所属:
出版社, 出版地: Katlenburg-Lindau, Germany : European Geophysical Society, Copernicus Publ.
ページ: 23 巻号: 17 通巻号: - 開始・終了ページ: - 識別子(ISBN, ISSN, DOIなど): ISSN: 1680-7367
CoNE: https://pure.mpg.de/cone/journals/resource/111076360006006