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  Electrocatalytic synthesis of hydrogen peroxide on Au–Pd nanoparticles: From fundamentals to continuous production

Pizzutilo, E., Kasian, O., Choi, C. H., Cherevko, S., Hutchings, G. J., Mayrhofer, K. J. J., et al. (2017). Electrocatalytic synthesis of hydrogen peroxide on Au–Pd nanoparticles: From fundamentals to continuous production. Chemical Physics Letters, 683, 436-442. doi:10.1016/j.cplett.2017.01.071.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-C5D2-D Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-C5D3-B
Genre: Journal Article

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 Creators:
Pizzutilo, Enrico1, Author              
Kasian, Olga1, Author              
Choi, Chang Hyuck1, 2, Author              
Cherevko, Serhiy1, 3, Author              
Hutchings, Graham J.4, Author              
Mayrhofer, Karl J. J.1, 3, 5, Author              
Freakley, Simon J.4, Author              
Affiliations:
1Electrocatalysis, Interface Chemistry and Surface Engineering, Max-Planck-Institut für Eisenforschung GmbH, Max Planck Society, ou_1863354              
2School of Materials Science and Engineering, Gwangju Institute of Science and Technology, Gwangju, South Korea, persistent22              
3Helmholtz-Institute Erlangen-Nuremberg for Renewable Energy (IEK-11), Forschungszentrum Jülich, Egerlandstrasse 3, 91058 Erlangen, Germany, ou_persistent22              
4Cardiff Catalysis Institute, School of Chemistry, Cardiff University, Main Building, Park Place, Cardiff, UK, persistent22              
5Department of Chemical and Biological Engineering, Friedrich-Alexander-Universität Erlangen-Nürnberg, 91058 Erlangen, Germany , ou_persistent22              

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Free keywords: PALLADIUM-GOLD ALLOYS; OXYGEN REDUCTION; H2O2 PRODUCTION; FUEL-CELL; SELECTIVITY; PLATINUM; SURFACE; ELECTROREDUCTION; NANOALLOYS; ELECTRODES;
 Abstract: The electrochemical synthesis of hydrogen peroxide (H2O2) represents a promising alternative to the anthraquinone process, as it combines on-site chemical and electrical production. The design of selective electrocatalysts is challenging and is commonly based on the alloying of elements to generate a synergistic effect and increase activity. In the present work, we report the electrochemical activity of Au-Pd nanoparticles immobilized directly onto an electrode as a model to study H2O2 electrochemical synthesis from fundamentals to continuous production. The impact of composition on the oxygen reduction reaction (ORR), the selectivity, as well as the peroxide reduction and oxidation reactions (PROR) are studied. (C) 2017 Elsevier B.V. All rights reserved.

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Language(s): eng - English
 Dates: 2017-09-01
 Publication Status: Published in print
 Pages: 7
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Degree: -

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Title: Chemical Physics Letters
  Other : Chem. Phys. Lett.
Source Genre: Journal
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Publ. Info: Amsterdam : North-Holland
Pages: - Volume / Issue: 683 Sequence Number: - Start / End Page: 436 - 442 Identifier: ISSN: 0009-2614
CoNE: /journals/resource/954925389241