Imaging molecular structure through femtosecond photoelectron diffraction on 
aligned and oriented gas-phase molecules

Boll, Rebecca; Rouzée, Arnaud; Adolph, Marcus; Anielski , Denis; Aquila, Andrew; Bari, Sadia; Bomme, Cédric; Bostedt, Christoph; Bozek, John D.; Chapman, Henry N.; Christensen, Lauge; Coffee, Ryan; Coppola, Niccola; De, Sankar; Decleva, Piero; Epp, Sascha; Erk, Benjamin; Filsinger, Frank; Foucar, Lutz; Gorkhover, Tais; Gumprecht, Lars; Hömke, André; Holmegaard, Lotte; Johnsson, Per; Kienitz, Jens S.; Kierspel, Thomas; Krasniqi, Faton; Kühnel, Kai-Uwe; Maurer, Jochen; Messerschmidt, Marc; Moshammer, Robert; Müller, Nele L. M.; Rudek, Benedikt; Savelyev, Evgeny; Schlichting, Ilme; Schmidt, Carlo; Scholz, Frank; Schorb, Sebastian; Schulz, Joachim; Seltmann, Jörn; Stener, Mauro; Stern, Stephan; Techert, Simone; Thøgersen, Jan; Trippel, Sebastian; Viefhaus, Jens; Vrakking, Marc; Stapelfeldt, Henrik; Küpper, Jochen; Ullrich, Joachim; Rudenko, Artem; Rolles, Daniel

doi:10.1039/C4FD00037D

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Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Boll, R., Rouzée, A., Adolph, M., Anielski, D., Aquila, A., Bari, S., et al. (2014). Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules. Faraday Discussions, 171, 57-80. doi:10.1039/C4FD00037D.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-F1CA-4 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-F1CB-2

Genre: Journal Article

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Boll, Rebecca^{1, 2, 3}, Author
Rouzée, Arnaud^{4, 5}, Author
Adolph, Marcus⁶, Author
Anielski , Denis^{1, 2, 3}, Author
Aquila, Andrew^{7, 8}, Author
Bari, Sadia⁸, Author
Bomme, Cédric¹, Author
Bostedt, Christoph⁹, Author
Bozek, John D.⁹, Author
Chapman, Henry N.^{7, 10, 11}, Author
Christensen, Lauge¹², Author
Coffee, Ryan⁹, Author
Coppola, Niccola^{7, 8}, Author
De, Sankar^{13, 14}, Author
Decleva, Piero¹⁵, Author
Epp, Sascha^{1, 2, 3, 16, 17}, Author
Erk, Benjamin^{1, 2, 3}, Author
Filsinger, Frank¹⁸, Author
Foucar, Lutz^{2, 19}, Author
Gorkhover, Tais⁶, Author
Gumprecht, Lars⁷, AuthorHömke, André^{1, 2}, AuthorHolmegaard, Lotte^{7, 13}, AuthorJohnsson, Per²⁰, AuthorKienitz, Jens S.^{7, 11}, AuthorKierspel, Thomas^{7, 11}, AuthorKrasniqi, Faton^{2, 7, 19}, AuthorKühnel, Kai-Uwe³, AuthorMaurer, Jochen¹³, AuthorMesserschmidt, Marc⁹, AuthorMoshammer, Robert^{2, 3}, AuthorMüller, Nele L. M.⁷, AuthorRudek, Benedikt^{2, 3, 21}, AuthorSavelyev, Evgeny^{1, 22}, AuthorSchlichting, Ilme¹⁹, AuthorSchmidt, Carlo^{2, 3}, AuthorScholz, Frank¹, AuthorSchorb, Sebastian⁹, AuthorSchulz, Joachim^{7, 8}, AuthorSeltmann, Jörn¹, AuthorStener, Mauro¹⁵, AuthorStern, Stephan^{7, 10}, AuthorTechert, Simone^{1, 2, 22, 23}, AuthorThøgersen, Jan¹³, AuthorTrippel, Sebastian⁷, AuthorViefhaus, Jens¹, AuthorVrakking, Marc^{4, 5}, AuthorStapelfeldt, Henrik¹³, AuthorKüpper, Jochen^{2, 7, 10, 11, 18}, AuthorUllrich, Joachim^{2, 3, 21}, AuthorRudenko, Artem^{2, 3, 24}, AuthorRolles, Daniel^{1, 2, 19}, Author more..

Affiliations:
1Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany, ou_persistent22
2Max Planck Advanced Study Group at CFEL, 22607 Hamburg, Germany, ou_persistent22
3Max Planck Institute for Nuclear Physics, 69117 Heidelberg, Germany, ou_persistent22
4Max-Born-Institut, 12489 Berlin, Germany, ou_persistent22
5FOM-Institute AMOLF, 1098 XG Amsterdam, The Netherlands, ou_persistent22
6Technische Universität Berlin, 10643 Berlin, Germany, ou_persistent22
7Center for Free-Electron Laser Science, DESY, 22607 Hamburg, Germany, ou_persistent22
8European XFEL GmbH, 22761 Hamburg, Germany, ou_persistent22
9SLAC National Accelerator Laboratory, Menlo Park, USA, ou_persistent22
10Department of Physics, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22
11Center for Ultrafast Imaging, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22
12Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22
13Department of Chemistry, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22
14Saha Institute of Nuclear Physics, 700064 Kolkata, India , ou_persistent22
15Dipartimento di Scienze Chimiche e Farmaceutiche, Università di Trieste, 34127 Trieste, Italy, ou_persistent22
16Max Planck Institute for Structural Dynamics, 22607 Hamburg, Germany, ou_persistent22
17Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938288
18Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545
19Max Planck Institute for Medical Research, 69120 Heidelberg, Germany, ou_persistent22
20Department of Physics, Lund University, 22100 Lund, Sweden, ou_persistent22
21Physikalisch-Technische Bundesanstalt (PTB), 38116 Braunschweig, Germany, ou_persistent22
22Institute of X-ray Physics, University, 37077 Göttingen, Germany, ou_persistent22
23Max Planck Institute for Biophysical Chemistry, 37077 Göttingen, Germany, ou_persistent22
24J.R. MacDonald Laboratory, Kansas State University, Manhattan, USA, ou_persistent22

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Abstract: This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump–probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C₈H₅F) and dissociating, laser-aligned 1,4-dibromobenzene (C₆H₄Br₂) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.

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Language(s): eng - English

Dates: Submitted: 2014-03-08Accepted: 2014-04-03Published Online: 2014-07-31Date issued: 2014-12-01

Publication Status: Issued

Pages: 24

Publishing info: -

Table of Contents: -

Rev. Type: Peer

Identifiers: DOI: 10.1039/C4FD00037D

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Title: Faraday Discussions

Source Genre: Journal

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Publ. Info: London : Royal Society of Chemistry

Pages: - Volume / Issue: 171 Sequence Number: - Start / End Page: 57 - 80 Identifier: ISSN: 1359-6640
CoNE: https://pure.mpg.de/cone/journals/resource/954925269326