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  Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules

Erk, B., Rolles, D., Foucar, L., Rudek, B., Epp, S., Cryle, M., et al. (2013). Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules. Physical Review Letters, 110(5): 53003, pp. 1-5. doi:10.1103/PhysRevLett.110.053003.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-F218-6 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-002D-F219-4
Genre: Journal Article
Alternative Title : Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules

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 Creators:
Erk, Benjamin1, Author
Rolles, Daniel1, Author
Foucar, Lutz1, Author
Rudek, Benedikt1, Author
Epp, Sascha2, Author              
Cryle, Max1, Author
Bostedt, Christoph, Author
Schorb, Sebastian, Author
Bozek, John D., Author
Rouzee, Arnaud, Author
Hundertmark, Axel, Author
Marchenko, Tatiana, Author
Simon, Marc, Author
Filsinger, Frank, Author
Christensen, Lauge, Author
De, Shankar, Author
Trippel, Sebastian, Author
Küpper, Jochen, Author
Stapelfeldt, Henrik, Author
Wada, Shinichi, Author
Ueda, Kiyoshi, AuthorSwiggers, Michelle L., AuthorMesserschmidt, Marc, AuthorSchroeter, Claus-Dieter, AuthorMoshammer, Robert, AuthorSchlichting, Ilme1, AuthorUllrich, Joachim, AuthorRudenko, Artem, Author more..
Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              
2Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society, ou_2025284              

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 Abstract: Ionization and fragmentation of methylselenol (CH(3)SeH) molecules by intense (>10(17) W/cm(2)) 5 fs x-ray pulses (ħω=2 keV) are studied by coincident ion momentum spectroscopy. We contrast the measured charge state distribution with data on atomic Kr, determine kinetic energies of resulting ionic fragments, and compare them to the outcome of a Coulomb explosion model. We find signatures of ultrafast charge redistribution from the inner-shell ionized Se atom to its molecular partners, and observe significant displacement of the atomic constituents in the course of multiple ionization.

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Language(s): eng - English
 Dates: 2012-10-022013-01-302013-01-302013-02-01
 Publication Status: Published in print
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Degree: -

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Title: Physical Review Letters
  Other : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 110 (5) Sequence Number: 53003 Start / End Page: 1 - 5 Identifier: ISSN: 0031-9007
CoNE: /journals/resource/954925433406_1