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  Influence of precursor porosity on sodium and sulfur promoted iron/carbon Fischer-Tropsch catalysts derived from metal-organic frameworks

Oschatz, M., Krause, S., Krans, N. A., Hernandez Mejia, C., Kaskel, S., & de Jong, K. P. (2017). Influence of precursor porosity on sodium and sulfur promoted iron/carbon Fischer-Tropsch catalysts derived from metal-organic frameworks. Chemical Communications, 53(73), 10204-10207. doi:10.1039/C7CC04877G.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002E-131C-1 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-002E-131D-0
Genre: Journal Article

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Oschatz, M.1, Author           
Krause, S., Author
Krans, N. A., Author
Hernandez Mejia, C., Author
Kaskel, S., Author
de Jong, K. P. , Author
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1External Organizations, ou_persistent22              

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 Abstract: Iron-based metal-organic frameworks (MOFs) with varying porosity are converted by pyrolysis into iron/carbon catalysts with predetermined composition and tailored pore structural features for the Fischer-Tropsch synthesis of lower C2-C4 olefins. Significantly higher activity arises for catalysts with higher porosity and decreased iron particle size derived from hierarchical MOF xerogel/aerogel precursors as compared to a purely microporous MOF. Post-synthetic functionalization using sodium and sulfur promoters further enhances the catalytic properties.

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 Dates: 2017
 Publication Status: Issued
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 Rev. Type: -
 Identifiers: DOI: 10.1039/C7CC04877G
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Title: Chemical Communications
  Other : Chem. Commun.
Source Genre: Journal
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: - Volume / Issue: 53 (73) Sequence Number: - Start / End Page: 10204 - 10207 Identifier: ISSN: 1359-7345