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  Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics.

Burt, M., Boll, R., Lee, J. W. L., Amini, K., Kockert, H., Vallance, C., et al. (2017). Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics. Physical Review A, 96(4): 043415. doi:10.1103/PhysRevA.96.043415.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-002E-1C44-C Version Permalink: http://hdl.handle.net/21.11116/0000-0001-1912-F
Genre: Journal Article

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 Creators:
Burt, M., Author
Boll, R., Author
Lee, J. W. L., Author
Amini, K., Author
Kockert, H., Author
Vallance, C., Author
Gentleman, A. S., Author
Mackenzie, S. R., Author
Bari, S., Author
Bomme, C., Author
Düsterer, S., Author
Erk, B., Author
Manschwetus, B., Author
Müller, E., Author
Rompotis, D., Author
Savelyev, E., Author
Schirmel, N., Author
Techert, S.1, Author              
Treusch, R., Author
Küpper, J., Author
Trippel, S., AuthorWiese, J., AuthorStapelfeldt, H., Authorde Miranda, B. C., AuthorGuillemin, R., AuthorIsmail, I., AuthorJournel, L., AuthorMarchenko, T., AuthorPalaudoux, J., AuthorPenent, F., AuthorPiancastelli, M. N., AuthorSimon, M., AuthorTravnikova, O., AuthorBrausse, F., AuthorGoldsztejn, G., AuthorRouzee, A., AuthorGeleoc, M., AuthorGeneaux, R., AuthorRuchon, T., AuthorUnderwood, J., AuthorHolland, D. M. P., AuthorMereshchenko, A. S., AuthorOlshin, P. K., AuthorJohnsson, P., AuthorMaclot, S., AuthorLahl, J., AuthorRudenko, A., AuthorZiaee, F., AuthorBrouard, M., AuthorRolles, D., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society, ou_578564              

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 Abstract: The dynamics following laser-induced molecular photodissociation of gas-phase CH2BrI at 271.6 nm were investigated by time-resolved Coulomb-explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH2BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of C(H)2Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb-explosion imaging as a real-time probe of chemical dynamics.

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Language(s): eng - English
 Dates: 2017-10-172017-10
 Publication Status: Published in print
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1103/PhysRevA.96.043415
 Degree: -

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Title: Physical Review A
Source Genre: Journal
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Publ. Info: -
Pages: 8 Volume / Issue: 96 (4) Sequence Number: 043415 Start / End Page: - Identifier: -