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  Severe pollution in China amplified by atmospheric moisture

Tie, X., Cao, J., Zhang, Q., Cheng, Y., Su, H., Chang, D., et al. (2017). Severe pollution in China amplified by atmospheric moisture. Scientific Reports. doi:10.1038/s41598-017-15909-1.

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 Urheber:
Tie, Xuexi, Autor
Cao, Junji, Autor
Zhang, Qiang, Autor
Cheng, Yafang1, Autor           
Su, Hang1, Autor           
Chang, Di1, Autor           
Pöschl, Ulrich1, Autor           
Hoffmann, Thorsten, Autor
Dusek, Uli, Autor
Li, Guohui, Autor
Worsnop, Douglas R., Autor
O'Dowd, Colin D., Autor
Affiliations:
1Multiphase Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826290              

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 Zusammenfassung: In recent years, severe haze events often occurred in China, causing serious environmental problems. The mechanisms responsible for the haze formation, however, are still not well understood, hindering the forecast and mitigation of haze pollution. Our study of the 2012–13 winter haze events in Beijing shows that atmospheric water vapour plays a critical role in enhancing the heavy haze events. Under weak solar radiation and stagnant moist meteorological conditions in winter, air pollutants and water vapour accumulate in a shallow planetary boundary layer (PBL). A positive feedback cycle is triggered resulting in the formation of heavy haze: (1) the dispersal of water vapour is constrained by the shallow PBL, leading to an increase in relative humidity (RH); (2) the high RH induces an increase of aerosol particle size by enhanced hygroscopic growth and multiphase reactions to increase particle size and mass, which results in (3) further dimming and decrease of PBL height, and thus further depressing of aerosol and water vapour in a very shallow PBL. This positive feedback constitutes a self-amplification mechanism in which water vapour leads to a trapping and massive increase of particulate matter in the near-surface air to which people are exposed with severe health hazards.

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Sprache(n): eng - English
 Datum: 2017
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1038/s41598-017-15909-1
 Art des Abschluß: -

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Titel: Scientific Reports
  Kurztitel : Sci. Rep.
Genre der Quelle: Zeitschrift
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Affiliations:
Ort, Verlag, Ausgabe: London, UK : Nature Publishing Group
Seiten: 8 Band / Heft: - Artikelnummer: - Start- / Endseite: - Identifikator: ISSN: 2045-2322
CoNE: https://pure.mpg.de/cone/journals/resource/2045-2322