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  Electron-phonon coupling constant of metallic overlayers from specular He atom scattering.

Benedek, G., Miret-Artés, S., Toennies, J. P., & Manson, J. R. (2018). Electron-phonon coupling constant of metallic overlayers from specular He atom scattering. The Journal of Physical Chemistry Letters, 9(1), 76-83. doi:10.1021/acs.jpclett.7b03047.

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Benedek, G., Author
Miret-Artés, S., Author
Toennies, Jan Peter1, Author           
Manson, J. R., Author
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1Emeritus Group Molecular Interactions, Max Planck Institute for Dynamics and Self-Organization, Max Planck Society, ou_2063297              

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 Abstract: He atom scattering has been shown to be a sensitive probe of electron− phonon interaction properties at surfaces. Here it is shown that measurements of the thermal attenuation of the specular He atom diffraction peak (the Debye−Waller effect) can determine the electron−phonon coupling constant, λ, for ultrathin films of metal overlayers on various close-packed metal substrates. Values of λ obtained for single and multiple monolayers of alkali metals, and for Pb layers on Cu(111), extrapolated to large thicknesses, agree favorably with known bulk values. This demonstrates that He atom scattering can measure the electron−phonon coupling strength as a function of film thickness on a layer-by-layer basis.

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Language(s): eng - English
 Dates: 2017-12-142018-01-04
 Publication Status: Issued
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 Rev. Type: Peer
 Identifiers: DOI: 10.1021/acs.jpclett.7b03047
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Title: The Journal of Physical Chemistry Letters
Source Genre: Journal
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Pages: - Volume / Issue: 9 (1) Sequence Number: - Start / End Page: 76 - 83 Identifier: -