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  Selective production of glycols from xylitol over Ru on covalent triazine frameworks - suppressing decarbonylation reactions

Beine, A. K., Krüger, A. J. D., Artz, J., Weidenthaler, C., Glotzbach, C., Hausoul, P. J. C., et al. (2018). Selective production of glycols from xylitol over Ru on covalent triazine frameworks - suppressing decarbonylation reactions. Green Chemistry, 20(6), 1316-1322. doi:10.1039/C8GC00208H.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-2BA5-5 Version Permalink: https://hdl.handle.net/21.11116/0000-0001-2BA6-4
Genre: Journal Article

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 Creators:
Beine, Anna Katharina1, Author
Krüger, Andreas J. D.1, Author
Artz, Jens1, Author
Weidenthaler, Claudia2, Author           
Glotzbach, Christoph3, Author
Hausoul, Peter J. C.1, Author
Palkovits, Regina1, Author
Affiliations:
1RWTH Aachen University, Worringerweg 2, 52074 Aachen, Germany , ou_persistent22              
2Research Group Weidenthaler, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1950291              
3Thyssenkrupp Industrial Solutions AG, ThyssenKrupp Allee 1, 45143 Essen, Germany, ou_persistent22              

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 Abstract: Ru on covaltent triazine frameworks (CTF) are highly active and selective catalysts for the conversion of xylitol to glycols (80% C-yield) in basic media. With increasing N-content decarbonylation reactions are suppressed leading to high glycol selectivity. The suppression can be attributed to the presence of N in the support and to metal-support interactions. The catalysts exhibit high stability and could be recycled 5 times with minor loss of activity.

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Language(s): eng - English
 Dates: 2018-01-192018-02-202018-02-232018-03-21
 Publication Status: Issued
 Pages: 7
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/C8GC00208H
 Degree: -

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Title: Green Chemistry
  Other : Green Chem.
Source Genre: Journal
 Creator(s):
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: - Volume / Issue: 20 (6) Sequence Number: - Start / End Page: 1316 - 1322 Identifier: ISSN: 1463-9262
CoNE: https://pure.mpg.de/cone/journals/resource/954925625301