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  Isotope and temperature effects in liquid water probed by x-ray absorption and resonant x-ray emission spectroscopy

Fuchs, O., Zharnikov, M., Weinhardt, L., Blum, M., Weigand, M., Zubavichus, Y., et al. (2008). Isotope and temperature effects in liquid water probed by x-ray absorption and resonant x-ray emission spectroscopy. Physical Review Letters, 100: 027801, pp. 1-4. doi:10.1103/PhysRevLett.100.027801.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-9917-9 Version Permalink: https://hdl.handle.net/21.11116/0000-0001-9918-8
Genre: Journal Article

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PhysRevLett_100_2008_027801.pdf (Any fulltext), 234KB
 
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https://journals.aps.org/prl/pdf/10.1103/PhysRevLett.100.027801 (Any fulltext)
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https://doi.org/10.1103/PhysRevLett.100.027801 (Any fulltext)
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 Creators:
Fuchs, O., Author
Zharnikov, M., Author
Weinhardt, L., Author
Blum, M., Author
Weigand, M., Author
Zubavichus, Y., Author
Bär, M., Author
Maier, F., Author
Denlinger, J. D., Author
Heske, C., Author
Grunze, Michael1, Author           
Umbach, E., Author
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              

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 Abstract: High-resolution x-ray absorption and emission spectra of liquid water exhibit a strong isotope effect. Further, the emission spectra show a splitting of the 1b1 emission line, a weak temperature effect, and a pronounced excitation-energy dependence. They can be described as a superposition of two independent contributions. By comparing with gas phase, ice, and NaOH/NaOD, we propose that the two components are governed by the initial state hydrogen bonding configuration and ultrafast dissociation on the time scale of the O 1s core hole decay.

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Language(s): eng - English
 Dates: 2007-03-102008-01-162008-01-16
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.100.027801
URI: https://www.ncbi.nlm.nih.gov/pubmed/18232928
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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 100 Sequence Number: 027801 Start / End Page: 1 - 4 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1