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  Nanofluidic ions transport and energy conversion through ultrathin free-standing polymeric carbon nitride membranes.

Xiao, K., Giusto, P., Wen, L., Jiang, L., & Antonietti, M. (2018). Nanofluidic ions transport and energy conversion through ultrathin free-standing polymeric carbon nitride membranes. Angewandte Chemie International Edition, 57(32), 10123-10126. doi:10.1002/anie.201804299.

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 Creators:
Xiao, Kai1, Author              
Giusto, Paolo2, Author              
Wen, Liping, Author
Jiang, Lei, Author
Antonietti, Markus3, Author              
Affiliations:
1Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              
2Paolo Giusto, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_3245192              
3Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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Free keywords: ions transport, carbon nitride, 2D membrane, nanoporous membrane, energy conversion
 Abstract: Ions transport through confined space with characteristic dimensions comparable to the Debye length has many applications, e.g. in water desalination, dialysis, and energy conversion. However, the existing 2D/3D smart porous membrane for ions transport and further applications are always fragile, thermolabile, and/or difficult to scale up, limiting their practical applicability. Here, we report that polymeric carbon nitride alternatively allows creating an ultrathin free-standing carbon nitride membrane (UFSCNM), which can be fabricated by simple CVD polymerization and exhibits per se excellent nanofluidic ions transport properties. The surface-charge-governed ion transport also endows such UFSCNMs with the function of converting salinity gradients into electric energy. With advantages of low cost, facile fabrication, and the ease of scale up while supporting high ionic currents, UFSCNM can be considered as an alternative candidate for the energy conversion system and new ionic devices.

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Language(s): eng - English
 Dates: 2018-06-252018
 Publication Status: Published in print
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Title: Angewandte Chemie International Edition
  Abbreviation : Angew. Chem., Int. Ed.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 57 (32) Sequence Number: - Start / End Page: 10123 - 10126 Identifier: ISSN: 1433-7851

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Title: Angewandte Chemie
  Abbreviation : Angew. Chem.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 130 (32) Sequence Number: - Start / End Page: 10280 - 10283 Identifier: ISSN: 0044-8249