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  Oxygen K-edge X-ray absorption fine structure studies of vacuum-deposited ice films

Zubavichus, Y., Zharnikov, M., Yang, Y.-J., Fuchs, O., Umbach, E., Heske, C., et al. (2006). Oxygen K-edge X-ray absorption fine structure studies of vacuum-deposited ice films. Langmuir, 22(17), 7241-7247. doi:10.1021/la060379o.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-9EDC-6 Version Permalink: https://hdl.handle.net/21.11116/0000-000A-127C-7
Genre: Journal Article

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 Creators:
Zubavichus, Yan, Author
Zharnikov, Michael, Author
Yang, Yong-Jie, Author
Fuchs, Oliver, Author
Umbach, Eberhard, Author
Heske, Clemens, Author
Grunze, Michael1, Author           
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              

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 Abstract: Multilayer ice films deposited on polycrystalline Au(111) substrates at 90 and 153 K under ultra-high-vacuum conditions are studied using O K-edge X-ray absorption fine structure spectroscopy in the surface-sensitive partial electron yield mode. Both near-edge and extended oscillatory fine structures are analyzed in combination with the theoretical real-space full-multiple-scattering simulations based on the FEFF8 code. The experimental data consistently indicate that the local structure of the near-surface regions in ice films at both substrate temperatures resembles that of high-density crystalline modifications of ice (e.g., ice II, ice III, or high-density amorphous ice). In addition, the ice films deposited at 153 K most probably contain a minor fraction of low-density cubic ice (Ic phase).

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Language(s): eng - English
 Dates: 2006-02-082006-05-082006-07-19
 Publication Status: Issued
 Pages: 7
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/la060379o
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Title: Langmuir
Source Genre: Journal
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Publ. Info: Columbus, OH : American Chemical Society
Pages: - Volume / Issue: 22 (17) Sequence Number: - Start / End Page: 7241 - 7247 Identifier: ISSN: 0743-7463
CoNE: https://pure.mpg.de/cone/journals/resource/954925541194