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  Surface chemistry of ultrathin films of histidine on gold as probed by high-resolution synchrotron photoemission

Zubavichus, Y., Zharnikov, M., Yang, Y., Fuchs, O., Heske, C., Umbach, E., et al. (2004). Surface chemistry of ultrathin films of histidine on gold as probed by high-resolution synchrotron photoemission. The Journal of Physical Chemistry B, 109(2), 884-891. doi:10.1021/jp047626m.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-ABAF-A Version Permalink: https://hdl.handle.net/21.11116/0000-0001-ABB0-7
Genre: Journal Article

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JPhysChemB_109_2005_884.pdf (Any fulltext), 238KB
 
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https://pubs.acs.org/doi/pdf/10.1021/jp047626m (Any fulltext)
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https://doi.org/10.1021/jp047626m (Any fulltext)
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 Creators:
Zubavichus, Yan, Author
Zharnikov, Michael, Author
Yang, Yongjie, Author
Fuchs, Oliver, Author
Heske, Clemens, Author
Umbach, Eberhard, Author
Tzvetkov, George, Author
Netzer, Falko P., Author
Grunze, Michael1, Author           
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              

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 Abstract: Procedures for the vacuum deposition of thin histidine films on polycrystalline Au(111) and their characterization with high-resolution synchrotron-radiation-based photoelectron spectroscopy are reported. The chemical form of histidine (anionic vs zwitterionic) and the nature of its interactions with the substrate (strong ionic-covalent vs weak van der Waals bonding) in mono- and multilayer films are analyzed. It is shown that water adsorption on a pre-prepared histidine film at 100 K results in protonation of histidine molecules and partial formation of hydroxyl anions. These chemical effects are carefully differentiated from spectral changes associated with radiation damage of the histidine films.

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Language(s): eng - English
 Dates: 2004-06-022004-10-212004-12-03
 Publication Status: Issued
 Pages: 8
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/jp047626m
URN: https://www.ncbi.nlm.nih.gov/pubmed/16866455
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Title: The Journal of Physical Chemistry B
  Other : J. Phys. Chem. B
Source Genre: Journal
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Publ. Info: Washington, D.C. : American Chemical Society
Pages: - Volume / Issue: 109 (2) Sequence Number: - Start / End Page: 884 - 891 Identifier: ISSN: 1520-6106
CoNE: https://pure.mpg.de/cone/journals/resource/1000000000293370_1