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  Setting the photoelectron clock through molecular alignment

Trabattoni, A., Wiese, J., de Giovannini, U., Olivieri, J.-F., Mullins, T., Onvlee, J., et al. (2020). Setting the photoelectron clock through molecular alignment. Nature Communications, 11(1): 2546. doi:10.1038/s41467-020-16270-0.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0001-B02B-8 Version Permalink: http://hdl.handle.net/21.11116/0000-0006-8AE7-A
Genre: Journal Article

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https://arxiv.org/abs/1802.06622 (Preprint)
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https://dx.doi.org/10.1038/s41467-020-16270-0 (Publisher version)
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 Creators:
Trabattoni, A.1, 2, Author
Wiese, J.1, 3, Author
de Giovannini, U.4, 5, Author              
Olivieri, J.-F.1, Author
Mullins, T.1, Author
Onvlee, J.1, Author
Son, S.-K.1, 2, Author
Frusteri, B.6, Author
Rubio, A.4, 7, 8, Author              
Trippel, S.1, 2, Author
Küpper, J.1, 2, 3, 8, Author
Affiliations:
1Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, ou_persistent22              
2The Hamburg Center forUltrafast Imaging, Universität Hamburg, ou_persistent22              
3Department of Chemistry, Universität Hamburg, ou_persistent22              
4Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
5Center for Free-Electron Laser Science, ou_persistent22              
6Dipartimento di Fisica e Chimica, Universitá degli Studi di Palermo, ou_persistent22              
7Center for Computational Quantum Physics (CCQ), The Flatiron Institute, ou_persistent22              
8Department of Physics, Universität Hamburg, ou_persistent22              

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 Abstract: The interaction of strong laser fields with matter intrinsically provides a powerful tool for imaging transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules, and show a full real-time picture of the photoelectron dynamics in the combined action of the laser field and the molecular interaction. We demonstrate that the molecule has a dramatic impact on the overall strong-field dynamics: it sets the clock for the emission of electrons with a given rescattering kinetic energy. This result represents a benchmark for the seminal statements of molecular-frame strong-field physics and has strong impact on the interpretation of self-diffraction experiments. Furthermore, the resulting encoding of the time-energy relation in molecular-frame photoelectron momentum distributions shows the way of probing the molecular potential in real-time, and accessing a deeper understanding of electron transport during strong-field interactions.

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Language(s): eng - English
 Dates: 2020-02-282020-04-162020-05-21
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: arXiv: 1802.06622
DOI: 10.1038/s41467-020-16270-0
 Degree: -

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Project name : -
Grant ID : 614507
Funding program : Funding Programme 7 (FP7)
Funding organization : European Commission (EC)
Project name : -
Grant ID : 694097
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

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Title: Nature Communications
  Abbreviation : Nat. Commun.
Source Genre: Journal
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Publ. Info: London : Nature Publishing Group
Pages: - Volume / Issue: 11 (1) Sequence Number: 2546 Start / End Page: - Identifier: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723