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  The effect of electrostatic fields on an oligo(ethylene glycol) terminated alkanethiol self-assembled monolayer

Pertsin, A. J., Grunze, M., Kreuzer, H. J., & Wang, R. L. C. (2000). The effect of electrostatic fields on an oligo(ethylene glycol) terminated alkanethiol self-assembled monolayer. Physical Chemistry Chemical Physics, 2(8), 1729-1733. doi:10.1039/B001293I.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-BA5B-8 Version Permalink: https://hdl.handle.net/21.11116/0000-0001-BA68-9
Genre: Journal Article

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PhysChemChemPhys_2_2000_1729.pdf (Any fulltext), 221KB
 
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http://pubs.rsc.org/en/content/articlepdf/2000/cp/b001293i (Any fulltext)
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 Creators:
Pertsin, Alexander J., Author
Grunze, Michael1, Author           
Kreuzer, H. Jürgen, Author
Wang, Richard L. C., Author
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              

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 Abstract: Static energy minimization and Monte Carlo simulation are used to study the effect of external electrostatic fields on the structure of a self-assembled monolayer (SAM) formed by methoxytri(ethylene glycol) terminated alkanethiol molecules. It is found that fields of the order of 1 V Å−1 in strength can substantially change the equilibrium configuration of the SAM, making the oxygen atoms of the terminal methoxy groups buried or exposed depending on the field polarity, which is qualitatively similar to what was found in our previous ab initio calculations with a single molecule. This finding implies a potential possibility of developing SAM-coated surfaces with electrically controlled (switchable) properties.

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Language(s): eng - English
 Dates: 1999-12-062000-02-172000
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/B001293I
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Title: Physical Chemistry Chemical Physics
  Abbreviation : Phys. Chem. Chem. Phys.
Source Genre: Journal
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Publ. Info: Cambridge, England : Royal Society of Chemistry
Pages: - Volume / Issue: 2 (8) Sequence Number: - Start / End Page: 1729 - 1733 Identifier: ISSN: 1463-9076
CoNE: https://pure.mpg.de/cone/journals/resource/954925272413_1