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  Peptides as Versatile Platforms for Quantum Computing

Rosaleny, L. E., Salvador, C.-S., Escalera-Moreno, L., Baldovi, J., Gołȩbiewska, V., Wlazło, K., et al. (2018). Peptides as Versatile Platforms for Quantum Computing. The Journal of Physical Chemistry Letters, 9(16), 4522-4526. doi:10.1021/acs.jpclett.8b01813.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-DE2E-3 Version Permalink: https://hdl.handle.net/21.11116/0000-0006-D57A-1
Genre: Journal Article

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Supporting information. - Additional information on several experimental and theoretical details and also on future perspectives, a spectroscopic characterization, additional CW EPR and pulsed EPR experimental characterization, considerations related to folding patterns (SHAPE), and a summary of the crystallization efforts
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https://dx.doi.org/10.1021/acs.jpclett.8b01813 (Publisher version)
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 Creators:
Rosaleny, L. E.1, Author
Salvador, C.-S.1, Author
Escalera-Moreno, L.1, Author
Baldovi, J.2, Author           
Gołȩbiewska, V.1, Author
Wlazło, K.1, Author
Casino, P.3, Author
Prima-García, H.1, Author
Gaita-Ariño, A.1, Author
Coronado, E.1, Author
Affiliations:
1Institut de Ciència Molecular, Universitat de València, ou_persistent22              
2Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
3Departamento de Bioquı́mica y Biologı́a Molecular, ERI BioTecMed, Universitat de València, ou_persistent22              

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 Abstract: The pursuit of novel functional building blocks for the emerging field of quantum computing is one of the most appealing topics in the context of quantum technologies. Herein we showcase the urgency of introducing peptides as versatile platforms for quantum computing. In particular, we focus on lanthanide-binding tags, originally developed for the study of protein structure. We use pulsed electronic paramagnetic resonance to demonstrate quantum coherent oscillations in both neodymium and gadolinium peptidic qubits. Calculations based on density functional theory followed by a ligand field analysis indicate the possibility of influencing the nature of the spin qubit states by means of controlled changes in the peptidic sequence. We conclude with an overview of the challenges and opportunities opened by this interdisciplinary field.

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Language(s): eng - English
 Dates: 2018-06-112018-07-252018-07-252018-08-16
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/acs.jpclett.8b01813
 Degree: -

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Project name : The present work has been funded by the EU (ERC Consolidator Grant 647301 DECRESIM, ERC Advanced Grant 788222 Mol-2D, and COST 15128 Molecular Spintronics Project), th e Spanish MINECO (grants MAT2017-89528 and CTQ2017-89993 co fi nanced by FEDER and Excellence Unit Mar ı ́ a de Maeztu MDM-2015- 0538), and the Generalitat Valenciana (Prometeo Program of Excellence). A.G.-A. acknowledges funding by the MINECO (Ramo ́ n y Cajal Program), L.E.-M. thanks the Generalitat Valenciana for a VALi+d predoctoral grant. J.J.B. thanks the EU for a Marie Curie Fellowship (H2020-MSCA-IF-2016- 751047). S.C.-S. thanks the Spanish MINECO for a Juan de la Cierva Incorporacio ́ n postdoctoral Fellowship. We thank Samuel Man ̃ as-Valero and Jose ́ V. Usagre for their assistance in the preparation of the EPR samples.
Grant ID : 751047
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

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Title: The Journal of Physical Chemistry Letters
  Abbreviation : J. Phys. Chem. Lett.
Source Genre: Journal
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Publ. Info: Washington, DC : American Chemical Society
Pages: - Volume / Issue: 9 (16) Sequence Number: - Start / End Page: 4522 - 4526 Identifier: CoNE: https://pure.mpg.de/cone/journals/resource/1948-7185