Deutsch
 
Hilfe Datenschutzhinweis Impressum
  DetailsucheBrowse

Datensatz

DATENSATZ AKTIONENEXPORT
  Polarization-state-resolved high-harmonic spectroscopy of solids

Klemke, N., Tancogne-Dejean, N., Rossi, G. M., Yang, Y., Scheiba, F., Mainz, R. E., et al. (2019). Polarization-state-resolved high-harmonic spectroscopy of solids. Nature Communications, 10: 1319. doi:10.1038/s41467-019-09328-1.

Item is

Basisdaten

einblenden: ausblenden:
Genre: Zeitschriftenartikel

Dateien

einblenden: Dateien
ausblenden: Dateien
:
s41467-019-09328-1.pdf (Verlagsversion), 2MB
Name:
s41467-019-09328-1.pdf
Beschreibung:
This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.
OA-Status:
Keine Angabe
Sichtbarkeit:
Öffentlich
MIME-Typ / Prüfsumme:
application/pdf / [MD5]
Technische Metadaten:
Copyright Datum:
2019
Copyright Info:
© the Author(s)
:
41467_2019_9328_MOESM1_ESM.pdf (Ergänzendes Material), 4MB
Name:
41467_2019_9328_MOESM1_ESM.pdf
Beschreibung:
Supplementary Information
OA-Status:
Keine Angabe
Sichtbarkeit:
Öffentlich
MIME-Typ / Prüfsumme:
application/pdf / [MD5]
Technische Metadaten:
Copyright Datum:
2019
Copyright Info:
© the Author(s)
Lizenz:
-
:
41467_2019_9328_MOESM2_ESM.pdf (Ergänzendes Material), 69KB
Name:
41467_2019_9328_MOESM2_ESM.pdf
Beschreibung:
Peer Review File
OA-Status:
Keine Angabe
Sichtbarkeit:
Öffentlich
MIME-Typ / Prüfsumme:
application/pdf / [MD5]
Technische Metadaten:
Copyright Datum:
-
Copyright Info:
-
Lizenz:
-

Externe Referenzen

einblenden:
ausblenden:
externe Referenz:
https://arxiv.org/abs/1805.10453 (Preprint)
Beschreibung:
-
OA-Status:
Keine Angabe
externe Referenz:
https://dx.doi.org/10.1038/s41467-019-09328-1 (Verlagsversion)
Beschreibung:
-
OA-Status:
Keine Angabe

Urheber

einblenden:
ausblenden:
 Urheber:
Klemke, N.1, 2, Autor
Tancogne-Dejean, N.1, 3, Autor           
Rossi, G. M.1, 2, Autor
Yang, Y.1, 2, Autor
Scheiba, F.1, 2, Autor
Mainz, R. E.1, 2, Autor
Di Sciacca, G.1, Autor
Rubio, A.1, 2, 3, 4, 5, Autor           
Kärtner, F. X.1, 2, 4, Autor
Mücke, O. D.1, 4, Autor
Affiliations:
1Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, ou_persistent22              
2Physics Department, University of Hamburg, ou_persistent22              
3Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
4The Hamburg Centre for Ultrafast Imaging, ou_persistent22              
5Center for Computational Quantum Physics (CCQ), The Flatiron Institute, ou_persistent22              

Inhalt

einblenden:
ausblenden:
Schlagwörter: -
 Zusammenfassung: Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the fast carrier dynamics in crystals holds great promise for next-generation petahertz electronics and devices. The carrier dynamics can produce high-order harmonics of the driving field extending up into the extreme-ultraviolet region. Here, we introduce polarization-state-resolved high-harmonic spectroscopy of solids, which provides deeper insights into both electronic and structural sub-cycle dynamics. Performing high-harmonic generation measurements from silicon and quartz, we demonstrate that the polarization states of the harmonics are not only determined by crystal symmetries, but can be dynamically controlled, as a consequence of the intertwined interband and intraband electronic dynamics. We exploit this symmetry-dynamics duality to efficiently generate coherent circularly polarized harmonics from elliptically polarized pulses. Our experimental results are supported by ab-initio simulations, providing evidence for the microscopic origin of the phenomenon.

Details

einblenden:
ausblenden:
Sprache(n): eng - English
 Datum: 2019-01-172019-03-012019-03-21
 Publikationsstatus: Online veröffentlicht
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: arXiv: 1805.10453
DOI: 10.1038/s41467-019-09328-1
 Art des Abschluß: -

Veranstaltung

einblenden:

Entscheidung

einblenden:

Projektinformation

einblenden: ausblenden:
Projektname : -
Grant ID : 676580
Förderprogramm : Horizon 2020 (H2020)
Förderorganisation : European Commission (EC)
Projektname : We acknowledge support by the cluster of excellence “Advanced Imaging of Matter” (EXC 2056—project ID 390715994) and the priority program QUTIF (SPP1840 SOLSTICE) of the Deutsche Forschungsgemeinschaft, as well as financial support from the European Research Council (ERC-2015-AdG-694097), Grupos Consolidados (IT578-13), and European Union’s H2020 program under GA no. 676580 (NOMAD). N.T.-D., A.R., and O.D.M. thank M. Altarelli for very fruitful discussion. We thank M. Spiwek for help with the Laue X-ray diffraction characterization of samples.
Grant ID : -
Förderprogramm : -
Förderorganisation : -

Quelle 1

einblenden:
ausblenden:
Titel: Nature Communications
  Kurztitel : Nat. Commun.
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: London : Nature Publishing Group
Seiten: - Band / Heft: 10 Artikelnummer: 1319 Start- / Endseite: - Identifikator: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723