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  Polarization-state-resolved high-harmonic spectroscopy of solids

Klemke, N., Tancogne-Dejean, N., Rossi, G. M., Yang, Y., Scheiba, F., Mainz, R. E., et al. (2019). Polarization-state-resolved high-harmonic spectroscopy of solids. Nature Communications, 10: 1319. doi:10.1038/s41467-019-09328-1.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0002-4E5E-F Version Permalink: http://hdl.handle.net/21.11116/0000-0004-AA73-B
Genre: Journal Article

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https://arxiv.org/abs/1805.10453 (Preprint)
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 Creators:
Klemke, N.1, 2, Author
Tancogne-Dejean, N.1, 3, Author              
Rossi, G. M.1, 2, Author
Yang, Y.1, 2, Author
Scheiba, F.1, 2, Author
Mainz, R. E.1, 2, Author
Di Sciacca, G.1, Author
Rubio, A.1, 2, 3, 4, 5, Author              
Kärtner, F. X.1, 2, 4, Author
Mücke, O. D.1, 4, Author
Affiliations:
1Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, ou_persistent22              
2Physics Department, University of Hamburg, ou_persistent22              
3Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
4The Hamburg Centre for Ultrafast Imaging, ou_persistent22              
5Center for Computational Quantum Physics (CCQ), The Flatiron Institute, ou_persistent22              

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 Abstract: Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the fast carrier dynamics in crystals holds great promise for next-generation petahertz electronics and devices. The carrier dynamics can produce high-order harmonics of the driving field extending up into the extreme-ultraviolet region. Here, we introduce polarization-state-resolved high-harmonic spectroscopy of solids, which provides deeper insights into both electronic and structural sub-cycle dynamics. Performing high-harmonic generation measurements from silicon and quartz, we demonstrate that the polarization states of the harmonics are not only determined by crystal symmetries, but can be dynamically controlled, as a consequence of the intertwined interband and intraband electronic dynamics. We exploit this symmetry-dynamics duality to efficiently generate coherent circularly polarized harmonics from elliptically polarized pulses. Our experimental results are supported by ab-initio simulations, providing evidence for the microscopic origin of the phenomenon.

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Language(s): eng - English
 Dates: 2019-01-172019-03-012019-03-21
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: arXiv: 1805.10453
DOI: 10.1038/s41467-019-09328-1
 Degree: -

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Project name : We acknowledge support by the cluster of excellence “Advanced Imaging of Matter” (EXC 2056—project ID 390715994) and the priority program QUTIF (SPP1840 SOLSTICE) of the Deutsche Forschungsgemeinschaft, as well as financial support from the European Research Council (ERC-2015-AdG-694097), Grupos Consolidados (IT578-13), and European Union’s H2020 program under GA no. 676580 (NOMAD). N.T.-D., A.R., and O.D.M. thank M. Altarelli for very fruitful discussion. We thank M. Spiwek for help with the Laue X-ray diffraction characterization of samples.
Grant ID : 676580
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

Source 1

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Title: Nature Communications
  Abbreviation : Nat. Commun.
Source Genre: Journal
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Publ. Info: London : Nature Publishing Group
Pages: - Volume / Issue: 10 Sequence Number: 1319 Start / End Page: - Identifier: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723